School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing) , No.11, Xueyuan Road, Haidian District, Beijing 100083, China.
State Key Laboratory of Coal Resources and Safe Mining (CUMTB) , Beijing 100083, China.
Environ Sci Technol. 2017 Nov 7;51(21):12072-12080. doi: 10.1021/acs.est.7b01857. Epub 2017 Oct 10.
China, the largest coal producer in the world, is responsible for over 50% of the total global methane (CH) emissions from coal mining. However, the current emission inventory of CH4 from coal mining has large uncertainties because of the lack of localized emission factors (EFs). In this study, province-level CH4 EFs from coal mining in China were developed based on the data analysis of coal production and corresponding discharged CH4 emissions from 787 coal mines distributed in 25 provinces with different geological and operation conditions. Results show that the spatial distribution of CH EFs is highly variable with values as high as 36 m3/t and as low as 0.74 m3/t. Based on newly developed CH EFs and activity data, an inventory of the province-level CH4 emissions was built for 2005-2010. Results reveal that the total CH emissions in China increased from 11.5 Tg in 2005 to 16.0 Tg in 2010. By constructing a gray forecasting model for CH EFs and a regression model for activity, the province-level CH emissions from coal mining in China are forecasted for the years of 2011-2020. The estimates are compared with other published inventories. Our results have a reasonable agreement with USEPA's inventory and are lower by a factor of 1-2 than those estimated using the IPCC default EFs. This study could help guide CH mitigation policies and practices in China.
中国是世界上最大的煤炭生产国,其煤炭开采甲烷(CH)排放量占全球总量的 50%以上。然而,由于缺乏本地化的排放因子(EFs),当前煤炭开采甲烷排放量的排放清单存在很大的不确定性。在本研究中,根据中国 25 个省份 787 个煤矿的煤炭产量和相应的甲烷排放量数据进行了分析,开发了省级煤矿甲烷排放因子。结果表明,CH 排放因子的空间分布差异很大,其值高达 36m3/t,低至 0.74m3/t。基于新开发的 CH 排放因子和活动数据,建立了 2005-2010 年省级 CH4 排放清单。结果表明,中国的总 CH 排放量从 2005 年的 11.5Tg 增加到 2010 年的 16.0Tg。通过构建 CH 排放因子的灰色预测模型和活动回归模型,对 2011-2020 年中国煤矿开采 CH 排放量进行了预测。将预测结果与其他已发表的清单进行了比较。我们的结果与美国环保署的清单有较好的一致性,比使用 IPCC 默认排放因子的估计值低 1-2 倍。本研究可以为中国的 CH 减排政策和实践提供指导。