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单层二硫化钼中的激子霍尔效应

Exciton Hall effect in monolayer MoS.

作者信息

Onga Masaru, Zhang Yijin, Ideue Toshiya, Iwasa Yoshihiro

机构信息

Quantum-Phase Electronics Center (QPEC) and Department of Applied Physics, The University of Tokyo, Tokyo 113-8656, Japan.

The Institute of Scientific and Industrial Research, Osaka University, Osaka 067-0047, Japan.

出版信息

Nat Mater. 2017 Dec;16(12):1193-1197. doi: 10.1038/nmat4996. Epub 2017 Oct 2.

Abstract

The spontaneous Hall effect driven by the quantum Berry phase (which serves as an internal magnetic flux in momentum space) manifests the topological nature of quasiparticles and can be used to control the information flow, such as spin and valley. We report a Hall effect of excitons (fundamental composite particles of electrons and holes that dominate optical responses in semiconductors). By polarization-resolved photoluminescence mapping, we directly observed the Hall effect of excitons in monolayer MoS and valley-selective spatial transport of excitons on a micrometre scale. The Hall angle of excitons is found to be much larger than that of single electrons in monolayer MoS (ref. ), implying that the quantum transport of the composite particles is significantly affected by their internal structures. The present result not only poses a fundamental problem of the Hall effect in composite particles, but also offers a route to explore exciton-based valleytronics in two-dimensional materials.

摘要

由量子贝里相位驱动的自发霍尔效应(其在动量空间中充当内部磁通量)体现了准粒子的拓扑性质,并可用于控制信息流,如自旋和能谷。我们报道了激子(电子和空穴的基本复合粒子,在半导体中主导光学响应)的霍尔效应。通过偏振分辨光致发光映射,我们直接观测到了单层二硫化钼中激子的霍尔效应以及激子在微米尺度上的能谷选择性空间输运。发现激子的霍尔角比单层二硫化钼中单个电子的霍尔角大得多(参考文献),这意味着复合粒子的量子输运受到其内部结构的显著影响。目前的结果不仅提出了复合粒子中霍尔效应的一个基本问题,而且还提供了一条在二维材料中探索基于激子的谷电子学的途径。

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