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锆-89 产率的建模与实验数据

Modeling and experimental data of zirconium-89 production yield.

作者信息

Sharifian Mozhgan, Sadeghi Mahdi, Alirezapour Behrouz, Yarmohammadi Mohammad, Ardaneh Khosro

机构信息

Department of Physics, Payame Noor University, P.O. Box: 19395-3697, Tehran, Iran.

Medical physics department, School of Medicine, Iran University of Medical Science, P.O. Box: 14155-6183, Tehran, Iran.

出版信息

Appl Radiat Isot. 2017 Dec;130:206-210. doi: 10.1016/j.apradiso.2017.09.044. Epub 2017 Sep 29.

Abstract

The radionuclide zirconium-89 can be employed for the positron emission tomography (PET). In this study Zr excitation function via Y(p,n)Zr reaction was calculated by the TALYS-1.8 code based on microscopic level density model. The formation of Zr was simulated using the Monte Carlo simulation code MCNPX to calculate the integral yield in the Y target body for threshold up to 40MeV incident-proton energy. The target thickness was based on calculation of the stopping power using the SRIM-2013 code matched to any incident-proton energy. The production yield of the Zr simulated with the Monte Carlo method for the Y(p,n)Zr, Y(d,2n)Zr, Sr(α,xn)Zr and Zr(p,pxn)Zr reactions and the results were in good agreement with published experimental results for the optimum energy range. An experimental yield of 53.1MB/µA for the 15MeV proton-induced on YO powder as a disk-target obtained for 1h irradiation at the AMIRS cyclotron.

摘要

放射性核素锆 -89 可用于正电子发射断层扫描(PET)。在本研究中,基于微观能级密度模型,利用 TALYS - 1.8 代码计算了通过 Y(p,n)Zr 反应产生锆的激发函数。使用蒙特卡罗模拟代码 MCNPX 模拟锆的生成过程,以计算在入射质子能量阈值高达 40MeV 时 Y 靶体中的积分产额。靶体厚度基于使用与任何入射质子能量匹配的 SRIM - 2013 代码计算的阻止本领。用蒙特卡罗方法模拟的 Y(p,n)Zr、Y(d,2n)Zr、Sr(α,xn)Zr 和 Zr(p,pxn)Zr 反应中锆的产额,其结果与已发表的在最佳能量范围内的实验结果高度吻合。在 AMIRS 回旋加速器上,以 15MeV 质子束辐照 YO 粉末圆盘靶 1 小时,获得的实验产额为 53.1MB/µA。

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