Beijing Key Laboratory for Magneto-Photoelectrical Composite and Interface Science, Center for Green Innovation, School of Mathematics and Physics, University of Science and Technology Beijing , Beijing, 100083, People's Republic of China.
The Beijing Key Laboratory for Nano-Photonics and Nano-Structure, Center for Condensed Matter Physics, Department of Physics, Capital Normal University , Beijing 100048, People's Republic of China.
Langmuir. 2017 Oct 31;33(43):12102-12107. doi: 10.1021/acs.langmuir.7b03144. Epub 2017 Oct 19.
Revealing the nature of plasmon-exciton co-driven surface catalytic reactions is important and urgent for developing potential applications in energy and environmental science. In this work, we propose a mechanism for plasmon-exciton co-driven surface catalytic reactions based on our experimental results. We provide a method for a unified treatment for reduction and oxidation reactions, which not only strongly supports our proposed mechanism but also promotes a deeper understanding of plasmon-exciton co-driven surface catalytic reactions.
揭示等离子激元-激子协同驱动的表面催化反应的本质对于在能源和环境科学中开发潜在应用具有重要性和紧迫性。在这项工作中,我们根据实验结果提出了一种等离子激元-激子协同驱动的表面催化反应机制。我们提供了一种统一处理还原和氧化反应的方法,不仅强烈支持了我们提出的机制,而且促进了对等离子激元-激子协同驱动的表面催化反应的更深入理解。