Kale Akshay, Song Le, Lu Xinyu, Yu Liandong, Hu Guoqing, Xuan Xiangchun
Department of Mechanical Engineering, Clemson University, Clemson, USA.
School of Instrument Science and Opto-electronic Engineering, Hefei University of Technology, Hefei, P. R. China.
Electrophoresis. 2018 Mar;39(5-6):887-896. doi: 10.1002/elps.201700342. Epub 2017 Nov 14.
Insulator-based dielectrophoresis (iDEP) exploits in-channel hurdles and posts etc. to create electric field gradients for various particle manipulations. However, the presence of such insulating structures also amplifies the Joule heating in the fluid around themselves, leading to both temperature gradients and electrothermal flow. These Joule heating effects have been previously demonstrated to weaken the dielectrophoretic focusing and trapping of microscale and nanoscale particles. We find that the electrothermal flow vortices are able to entrain submicron particles for a localized enrichment near the insulating tips of a ratchet microchannel. This increase in particle concentration is reasonably predicted by a full-scale numerical simulation of the mass transport along with the coupled charge, heat and fluid transport. Our model also predicts the electric current and flow pattern in the fluid with a good agreement with the experimental observations.
基于绝缘体的介电泳(iDEP)利用通道内的障碍物和柱体等,为各种粒子操控创建电场梯度。然而,此类绝缘结构的存在也会放大其周围流体中的焦耳热,导致温度梯度和电热流。此前已证明,这些焦耳热效应会削弱介电泳对微米级和纳米级粒子的聚焦和捕获。我们发现,电热流涡旋能够夹带亚微米粒子,使其在棘轮微通道绝缘尖端附近局部富集。通过对质量传输以及耦合的电荷、热和流体传输进行全尺度数值模拟,合理地预测了粒子浓度的这种增加。我们的模型还预测了流体中的电流和流动模式,与实验观测结果吻合良好。