State Environmental Protection Scientific Observation and Research Station for Lake Dongtinghu (SEPSORSLD), National Engineering Laboratory for Lake Pollution Control and Ecological Restoration, State Key Laboratory of Environmental Criteria and Risk Assessment, Research Centre of Lake Environment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China.
School of Resources and Environment, Hefei University of Technology, Hefei, Anhui, 238000, China.
Environ Sci Pollut Res Int. 2018 Jan;25(3):2603-2613. doi: 10.1007/s11356-017-0332-4. Epub 2017 Nov 12.
According to current study, seven surface sediments and three sediment cores were collected from three typical areas of Tiaoxi River, which were living area, agricultural area, and industrial area. The water quantity into the Lake Taihu from the Tiaoxi River accounted for almost one third of the total water quantity by all rivers into the Lake Taihu. To study geochemical features and pollution history of heavy metals in three typical areas of Tiaoxi River, total content and chemical fractionations of Cu, Pb, Cd, Cr, Mn, Zn, Fe, As, and Hg were analyzed for surface and core sediments using the speciation extraction procedure, proposed by the Commission of the European Communities Bureau of Reference (BCR), together with grain size and organic carbon measurements. The results showed that the concentration of nine heavy metals and the variation characteristics of Zn, Cu, Fe, Mn, and Cr are different among five cores, which has shown that the river responses to natural and anthropogenic activities were dissimilar in various areas. BCR sequential extraction showed contents of Cr, Fe, and Cu were dominated in the remaining parts. Non-residual fractions for Zn and Mn contained major portions. Based on RAC (risk assessment core), the risk of Mn was high to very high in the three typical areas, and the risk of Zn was medium in the three typical areas.
根据目前的研究,从太湖南部的三条典型河流——漕桥河的生活区域、农业区和工业区——采集了七个表层沉积物和三个沉积物岩芯。漕桥河流入太湖的水量占所有入湖河流总水量的近三分之一。为了研究漕桥河三个典型区域的重金属地球化学特征和污染历史,采用欧盟委员会基准局(BCR)提出的分级提取程序,对表层和岩芯沉积物中的 Cu、Pb、Cd、Cr、Mn、Zn、Fe、As 和 Hg 的总含量和化学形态进行了分析,并结合粒度和有机碳测量。结果表明,五个岩芯中九种重金属的浓度和 Zn、Cu、Fe、Mn 和 Cr 的变化特征不同,这表明河流对自然和人为活动的响应在不同地区是不同的。BCR 连续提取表明 Cr、Fe 和 Cu 主要存在于残余部分。Zn 和 Mn 的非残余部分含量较大。基于 RAC(风险评估核心),三个典型区域的 Mn 风险为高至高,三个典型区域的 Zn 风险为中。