Optical Materials Engineering Laboratory, Department of Mechanical and Process Engineering, ETH Zurich , 8092 Zurich, Switzerland.
ACS Nano. 2017 Dec 26;11(12):12167-12173. doi: 10.1021/acsnano.7b05269. Epub 2017 Nov 30.
Combining the ability to localize electromagnetic fields at the nanoscale with a directional response, plasmonic antennas offer an effective strategy to shape the far-field pattern of coupled emitters. Here, we introduce a family of directional multiresonant antennas that allows for polarization-resolved spectral identification of fluorescent emission. The geometry consists of a central aperture surrounded by concentric polygonal corrugations. By varying the periodicity of each axis of the polygon individually, this structure can support multiple resonances that provide independent control over emission directionality for multiple wavelengths. Moreover, since each resonant wavelength is directly mapped to a specific polarization orientation, spectral information can be encoded in the polarization state of the out-scattered beam. To demonstrate the potential of such structures in enabling simplified detection schemes and additional functionalities in sensing and imaging applications, we use the central subwavelength aperture as a built-in nanocuvette and manipulate the fluorescent response of colloidal-quantum-dot emitters coupled to the multiresonant antenna.
将电磁场在纳米尺度上的局域化能力与定向响应相结合,等离子体激元天线为控制耦合发射器的远场模式提供了一种有效的策略。在这里,我们介绍了一系列定向多共振天线,它允许对荧光发射进行偏振分辨光谱识别。该几何形状由同心多边形波纹环绕的中心孔组成。通过单独改变多边形每条轴的周期性,该结构可以支持多个共振,从而为多个波长的发射方向性提供独立控制。此外,由于每个共振波长都直接映射到特定的偏振方向,因此光谱信息可以编码在出射光束的偏振态中。为了展示这种结构在简化传感和成像应用中的检测方案和附加功能方面的潜力,我们将亚波长中心孔用作内置纳米小室,并操纵与多共振天线耦合的胶体量子点发射器的荧光响应。