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彩虹辐射单晶 Ag 纳米线纳米天线。

Rainbow radiating single-crystal Ag nanowire nanoantenna.

机构信息

Department of Chemistry, KAIST, Daejeon 305-701, Korea.

出版信息

Nano Lett. 2012 May 9;12(5):2331-6. doi: 10.1021/nl3002414. Epub 2012 Apr 17.

Abstract

Optical antennas interface an object with optical radiation and boost the absorption and emission of light by the objects through the antenna modes. It has been much desired to enhance both excitation and emission processes of the quantum emitters as well as to interface multiwavelength channels for many nano-optical applications. Here we report the experimental implementation of an optical antenna operating in the full visible range via surface plasmon currents induced in a defect-free single-crystalline Ag nanowire (NW). With its atomically flat surface, the long Ag NW reliably establishes multiple plasmonic resonances and produces a unique rainbow antenna radiation in the Fresnel region. Detailed antenna radiation properties, such as radiating near-field patterns and polarization states, were experimentally examined and precisely analyzed by numerical simulations and antenna theory. The multiresonant Ag NW nanoantenna will find superb applications in nano-optical spectroscopy, high-resolution nanoimaging, photovoltaics, and nonlinear signal conversion.

摘要

光学天线将物体与光辐射连接起来,并通过天线模式增强物体对光的吸收和发射。人们一直希望增强量子发射器的激发和发射过程,并为许多纳米光学应用接口多波长通道。在这里,我们通过在无缺陷单晶 Ag 纳米线(NW)中感应表面等离激元电流,报告了一种在整个可见光范围内工作的光学天线的实验实现。由于其原子平坦的表面,长 Ag NW 可靠地建立了多个等离子体共振,并在菲涅尔区域产生独特的彩虹天线辐射。通过数值模拟和天线理论,对天线辐射特性(如辐射近场模式和偏振态)进行了详细的实验研究和精确分析。多共振 Ag NW 纳米天线将在纳米光学光谱学、高分辨率纳米成像、光伏和非线性信号转换等领域有极好的应用。

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