Department of Physics, Massachusetts Institute of Technology , Cambridge, Massachusetts 02139-4307, United States.
Department of Electrical Engineering and Solid State Institute, Technion , Haifa 3200008, Israel.
Nano Lett. 2018 Jan 10;18(1):308-313. doi: 10.1021/acs.nanolett.7b04146. Epub 2017 Dec 26.
Control over the spontaneous emission of light through tailored optical environments remains a fundamental paradigm in nanophotonics. The use of highly confined plasmons in materials such as graphene provides a promising platform to enhance transition rates in the IR-THz by many orders of magnitude. However, such enhancements involve near-field plasmon modes or other kinds of near-field coupling like quenching, and it is challenging to use these highly confined modes to harness light in the far-field due to the difficulty of plasmonic outcoupling. Here, we propose that through the use of radiative cascade chains in multilevel emitters, IR plasmons can be used to enhance far field spectra in the visible and UV range, even at energies greater than 10 eV. Combining Purcell-enhancement engineering, graphene plasmonics, and radiative cascade can result in a new type of UV emitter whose properties can be tuned by electrically doping graphene. Varying the distance between the emitter and the graphene surface can change the strength of the far-field emission lines by 2 orders of magnitude. We also find that the dependence of the far-field emission on the Fermi energy is potentially extremely sharp at the onset of interband transitions, allowing the Fermi energy to effectively serve as a "switch" for turning on and off certain plasmonic and far-field emissions.
通过定制光学环境来控制光的自发发射仍然是纳米光子学的基本范例。在诸如石墨烯之类的材料中使用高度受限的等离激元提供了一个有前途的平台,可以将 IR-THz 中的跃迁速率提高几个数量级。然而,这种增强涉及近场等离激元模式或其他类型的近场耦合,例如猝灭,由于等离子体激元的取出困难,因此难以利用这些高度受限的模式在远场中利用光。在这里,我们提出,通过在多级发射器中使用辐射级联链,可以使用 IR 等离激元来增强可见光和紫外范围内的远场光谱,即使在能量大于 10 eV 的情况下也是如此。结合 Purcell 增强工程、石墨烯等离激元和辐射级联,可以产生一种新型的 UV 发射器,其性质可以通过对石墨烯进行电掺杂来调节。改变发射器与石墨烯表面之间的距离可以使远场发射线的强度变化 2 个数量级。我们还发现,在带间跃迁开始时,远场发射对费米能的依赖性可能非常陡峭,这使得费米能有效地充当开启和关闭某些等离激元和远场发射的“开关”。