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用于增强可调谐红外等离子体激元的双层石墨烯

Double-layer graphene for enhanced tunable infrared plasmonics.

作者信息

Rodrigo Daniel, Tittl Andreas, Limaj Odeta, Abajo F Javier García de, Pruneri Valerio, Altug Hatice

机构信息

Institute of BioEngineering, École Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

ICFO-Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain.

出版信息

Light Sci Appl. 2017 Jun 2;6(6):e16277. doi: 10.1038/lsa.2016.277. eCollection 2017 Jun.

Abstract

Graphene is emerging as a promising material for photonic applications owing to its unique optoelectronic properties. Graphene supports tunable, long-lived and extremely confined plasmons that have great potential for applications such as biosensing and optical communications. However, in order to excite plasmonic resonances in graphene, this material requires a high doping level, which is challenging to achieve without degrading carrier mobility and stability. Here, we demonstrate that the infrared plasmonic response of a graphene multilayer stack is analogous to that of a highly doped single layer of graphene, preserving mobility and supporting plasmonic resonances with higher oscillator strength than previously explored single-layer devices. Particularly, we find that the optically equivalent carrier density in multilayer graphene is larger than the sum of those in the individual layers. Furthermore, electrostatic biasing in multilayer graphene is enhanced with respect to single layer due to the redistribution of carriers over different layers, thus extending the spectral tuning range of the plasmonic structure. The superior effective doping and improved tunability of multilayer graphene stacks should enable a plethora of future infrared plasmonic devices with high optical performance and wide tunability.

摘要

由于其独特的光电特性,石墨烯正成为一种有前途的光子应用材料。石墨烯支持可调谐、长寿命且高度受限的表面等离激元,在生物传感和光通信等应用中具有巨大潜力。然而,为了激发石墨烯中的表面等离激元共振,这种材料需要高掺杂水平,而在不降低载流子迁移率和稳定性的情况下实现这一点具有挑战性。在此,我们证明了石墨烯多层堆叠的红外表面等离激元响应类似于高度掺杂的单层石墨烯,保留了迁移率,并支持具有比先前探索的单层器件更高振子强度的表面等离激元共振。特别地,我们发现多层石墨烯中的光学等效载流子密度大于各层载流子密度之和。此外,由于载流子在不同层间的重新分布,多层石墨烯中的静电偏置相对于单层有所增强,从而扩展了表面等离激元结构的光谱调谐范围。多层石墨烯堆叠的卓越有效掺杂和改善的可调谐性应能使未来大量具有高光性能和宽可调谐性的红外表面等离激元器件成为可能。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d9b5/6062234/14874cae5d0e/lsa2016277f1.jpg

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