Mukherjee Debopreeti, Ortiz Rodriguez Lilliana I, Hilaire Mary Rose, Troxler Thomas, Gai Feng
Department of Chemistry University of Pennsylvania, 231 South 34th Street, Philadelphia, PA 19104, USA.
Phys Chem Chem Phys. 2018 Jan 28;20(4):2527-2535. doi: 10.1039/c7cp07160d. Epub 2018 Jan 9.
Considerable efforts have been devoted to the development of spectroscopic probes that are sensitive to water and can be used to monitor, for example, biological and chemical processes involving dehydration or hydration. Continuing this line of research, herein we show that 7-cyanoindole can serve as a sensitive fluorescence probe of hydration as its fluorescence properties, including intensity, peak wavelength and lifetime, depend on the amount of water in nine water-organic solvent mixtures. Our results indicate that 7-cyanoindole is not only able to reveal the underlying microheterogeneity of these binary solvent systems, but also offers distinct advantages. These include: (1) its fluorescence intensity increases more than ten times upon going from a hydrated to a dehydrated environment; (2) its peak wavelength shifts as much as 35 nm upon dehydration; (3) its single-exponential fluorescence decay lifetime increases from 2.0 ns in water to 8-16 ns in water-organic binary mixtures, making it viable to distinguish between differently hydrated environments via fluorescence lifetime measurements; and (4) its absorption spectrum is significantly red-shifted from that of indole, making selective excitation of its fluorescence possible in the presence of naturally occurring amino-acid fluorophores. Moreover, we find that for seven binary mixtures the fluorescence lifetimes of 7-cyanoindole measured at solvent compositions where maximum microheterogeneity occurs correlate linearly with the peak wavenumbers of its fluorescence spectra obtained in the respective pure organic solvents. This suggests that the microheterogeneities of these binary mixtures bear certain similarity, a phenomenon that warrants further investigation.
人们已经付出了相当大的努力来开发对水敏感的光谱探针,这些探针可用于监测,例如,涉及脱水或水合作用的生物和化学过程。延续这一研究方向,在此我们表明,7-氰基吲哚可作为一种对水合作用敏感的荧光探针,因为其荧光特性,包括强度、峰值波长和寿命,取决于九种水-有机溶剂混合物中的水量。我们的结果表明,7-氰基吲哚不仅能够揭示这些二元溶剂体系潜在的微观不均匀性,而且还具有明显的优势。这些优势包括:(包括:(1)从水合环境转变为脱水环境时,其荧光强度增加超过十倍;(2)脱水时其峰值波长移动多达35nm;(3)其单指数荧光衰减寿命从水中的2.0ns增加到水-有机二元混合物中的8-16ns,使得通过荧光寿命测量区分不同水合环境成为可能;(4)其吸收光谱相对于吲哚有明显的红移,使得在天然存在的氨基酸荧光团存在的情况下能够选择性地激发其荧光。此外,我们发现对于七种二元混合物,在出现最大微观不均匀性的溶剂组成下测量的7-氰基吲哚的荧光寿命与其在各自纯有机溶剂中获得的荧光光谱的峰值波数呈线性相关。这表明这些二元混合物的微观不均匀性具有一定的相似性,这一现象值得进一步研究。