Chemical & Biomolecular Engineering, Johns Hopkins University, Baltimore, MD 21218, USA.
Soft Matter. 2018 Feb 14;14(6):934-944. doi: 10.1039/c7sm02287e. Epub 2018 Jan 10.
We report a closed-form analytical model for energy landscapes of ellipsoidal particles in non-uniform high-frequency AC electric fields to identify all possible particle positions and orientations. Three-dimensional equilibrium positions and orientations of prolate (r = r < r), oblate (r = r > r), and scalene (r≠r≠r) ellipsoids are reported vs. field frequency and amplitude, which are determined from energy landscape minima. For ellipsoids within non-uniform electric fields between co-planar parallel electrodes, the number of configurations of position and orientation is 6 for prolate, 5 for oblate, and 9 for scalene ellipsoids. In addition, for coplanar electrodes, conditions are identified when particles can be treated using a quasi-2D analysis in the plane of their most probable elevation near an underlying surface. The reported expressions are valid for time-averaged interactions of ellipsoid particles in arbitrary AC electric field configurations, such that our results are applicable to electromagnetic tweezers interacting with particles having an appropriate material property contrast with the medium in the frequency range of interest.
我们提出了一种针对各向异性高频交流电场中椭球体能量景观的封闭解析模型,以确定所有可能的颗粒位置和取向。报告了在不同场频和场强下,各向异性椭球体(r = r < r 的扁长椭球体、r = r > r 的扁圆椭球体以及 r ≠ r ≠ r 的不等三轴椭球体)的三维平衡位置和取向,这些位置和取向是由能量景观最小值确定的。对于在共面平行电极之间的非均匀电场中的椭球体,扁长椭球体的位置和取向的配置数量为 6,扁圆椭球体的为 5,不等三轴椭球体的为 9。此外,对于共面电极,当颗粒在靠近下表面的最可能抬高平面内可以用准二维分析处理时,确定了相关条件。报告的表达式适用于任意交流电场配置中椭球体颗粒的时间平均相互作用,因此我们的结果适用于与感兴趣频率范围内的介质具有适当材料特性对比度的电磁镊子相互作用的颗粒。