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中国北京西南部污染农村地区气溶胶污染特征及其来源。

Characteristics and sources of aerosol pollution at a polluted rural site southwest in Beijing, China.

机构信息

State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China; State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China.

State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China; State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China.

出版信息

Sci Total Environ. 2018 Jun 1;626:519-527. doi: 10.1016/j.scitotenv.2018.01.047. Epub 2018 Feb 19.

Abstract

Annual average PM concentration in south Beijing was 30% and 40% higher than the whole Beijing city in 2015 and 2016, respectively. Few studies have been conducted to investigate what leads to the characteristics and sources of heavy pollution in the south rural area of Beijing. This study conducted an observation with Aerosol Chemical Speciation Monitor (ACSM) at a southwest rural site (Liulihe) in Beijing during 2014-2016, to investigate the seasonal aerosol characteristics and their sources. Positive matrix factorization (PMF) algorithm was used to distinguish different components of organic aerosol measured by ACSM. Biomass burning is an important pollution source, mainly due to the open burning after harvest season in autumn, regional transport in spring, and local residential biofuel use in winter. Coal consumption is the largest primary organic aerosol source in winter. Heavy duty diesel trucks contributed significantly to organic aerosol at night-time in the rural area. Results of this study show residential solid fuel burning is the most important source of aerosol pollution in the rural area of Beijing and the results focusing on urban Beijing might have underestimate the contribution from residential emissions in the Beijing-Tianjin-Hebei region.

摘要

2015 年和 2016 年,北京市南部地区年均 PM 浓度分别比全市高出 30%和 40%。针对导致北京市南部农村地区重污染特征和来源的问题,目前仅有少量研究开展。本研究于 2014 年至 2016 年在北京西南农村(琉璃河)设置观测点,利用气溶胶化学组分监测仪(ACSM)进行观测,以调查大气气溶胶的季节性特征及其来源。正矩阵因子化(PMF)算法用于区分 ACSM 测量的有机气溶胶的不同成分。生物质燃烧是一个重要的污染源,主要源自秋季收获后的露天焚烧、春季的区域传输,以及冬季当地居民使用生物燃料。煤炭消耗是冬季首要的原生有机气溶胶源。重型柴油卡车在农村地区夜间对有机气溶胶有显著贡献。本研究结果表明,居民固体燃料燃烧是北京市农村地区大气气溶胶污染的最重要来源,而仅关注北京市城区的结果可能低估了京津冀地区居民排放的贡献。

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