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中国东北农村地区总悬浮颗粒物中室内外多环芳烃(PAHs)污染特征:以供暖期和非供暖期为例

Characteristics of indoor and outdoor Polycyclic Aromatic Hydrocarbons (PAHs) pollution in TSP in rural Northeast China: A case study of heating and non-heating periods.

作者信息

Li Chunhui, Bai Li, Wang Han, Li Guangming, Cui Yongbo

机构信息

School of Municipal & Environmental Engineering, Jilin Jianzhu University, Changchun, 130118 China.

Key Laboratory of Songliao Aquatic of Education, Jilin Jianzhu University, Changchun, 130118 China.

出版信息

J Environ Health Sci Eng. 2022 Aug 23;20(2):899-913. doi: 10.1007/s40201-022-00830-1. eCollection 2022 Dec.

Abstract

Approximately 91% of the world's population lives in an air-polluted environment, and environmental pollution has become a widespread concern. Urban indoor and outdoor air pollution has been fully researched and effective control measures have been proposed. However, the issue of air pollution in rural areas has not been explored in depth. Compared to urban air pollution, the rural air pollution problem is more complex and urgent. Due to climatic factors and economic conditions in rural Northeast China, most households use solid fuels such as biomass straw and coal as domestic energy during the heating period, which will cause serious pollution problems of Total Suspended Particulate (TSP) and Polycyclic Aromatic Hydrocarbons (PAHs). To investigate the pollution characteristics of PAHs in indoor and outdoor TSP in rural Northeast China during the heating and non-heating periods, a medium-sized particulate matter collector 1108A was used to collect TSP for 7 days, and GC-MS was used to detect PAHs. The results showed that indoor TSP and PAHs pollution levels were the highest during the heating period. PAHs source analysis by Diagnostic Ratio (DR) and Principal Component Analysis (PCA) indicated that the main sources were biomass and coal combustion, vehicle emissions, and domestic waste incineration. According to the results of carcinogenic risk model calculations, there is a potential carcinogenic risk to the population in the Northeast rural living area. This study reflects the pollution characteristics and sources of indoor and outdoor TSP and PAHs in rural Northeast China during heating and non-heating periods, and provides a reference for further prevention and control of air pollution in rural areas, which is conducive to improving the living environment and improving human health.

摘要

全球约91%的人口生活在空气污染的环境中,环境污染已成为一个广泛关注的问题。城市室内和室外空气污染已得到充分研究,并已提出有效的控制措施。然而,农村地区的空气污染问题尚未得到深入探讨。与城市空气污染相比,农村空气污染问题更为复杂和紧迫。由于中国东北农村的气候因素和经济条件,大多数家庭在供暖期使用生物质秸秆和煤炭等固体燃料作为生活能源,这将导致总悬浮颗粒物(TSP)和多环芳烃(PAHs)严重污染问题。为了研究中国东北农村供暖期和非供暖期室内外TSP中PAHs的污染特征,使用中型颗粒物收集器1108A收集TSP 7天,并采用气相色谱-质谱联用仪检测PAHs。结果表明,供暖期室内TSP和PAHs污染水平最高。通过诊断比值(DR)和主成分分析(PCA)对PAHs源进行分析表明,主要来源是生物质和煤炭燃烧、车辆排放以及生活垃圾焚烧。根据致癌风险模型计算结果,中国东北农村居住地区人群存在潜在致癌风险。本研究反映了中国东北农村供暖期和非供暖期室内外TSP和PAHs的污染特征及来源,为农村地区进一步防治空气污染提供参考,有利于改善生活环境和增进人类健康。

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