Departmento de Ingeniería Química y Bioprocesos, Pontificia Universidad Católica de Chile, Avda. Vicuña Mackenna 4860, Santiago, 7820436, Chile.
Instituto de Geografía, Pontificia Universidad Católica de Chile, Avda. Vicuña Mackenna 4860, Santiago, 7820436, Chile.
Environ Pollut. 2018 May;236:477-487. doi: 10.1016/j.envpol.2018.01.085.
Temuco is a mid-size city representative of severe wood smoke pollution in southern Chile; however, little is known about the indoor air quality in this region. A field measurement campaign at 63 households in the Temuco urban area was conducted in winter 2014 and is reported here. In this study, indoor and outdoor (24-hr) PM and its elemental composition were measured and compared. Infiltration parameters and outdoor/indoor contributions to indoor PM were also determined. A statistical evaluation of how various air quality interventions and household features influence indoor PM was also performed. This study determined median indoor and outdoor PM concentrations of 44.4 and 41.8 μg/m, respectively. An average infiltration factor (0.62 ± 0.06) was estimated using sulfur as a tracer species. Using a simple mass balance approach, median indoor and outdoor contributions to indoor PM concentrations were then estimated as 12.5 and 26.5 μg/m, respectively; therefore, 68% of indoor PM comes from outdoor infiltration. This high percentage is due to high outdoor pollution and relatively high household air exchange rates (median: 1.06 h). This study found that S, Br and Rb were dominated by outdoor contributions, while Si, Ca, Ti, Fe and As originated from indoor sources. Using continuous indoor and outdoor PM measurements, a median indoor source strength of 75 μg PM/min was estimated for the diurnal period, similar to literature results. For the evening period, the median estimate rose to 135 μg PM/min, reflecting a more intense wood burning associated to cooking and space heating at night. Statistical test results (at the 90% confidence level) support the ongoing woodstove replacement program (reducing emissions) and household weatherization subsidies (reducing heating demand) for improving indoor air quality in southern Chile, and suggest that a cookstove improvement program might be helpful as well.
特木科是智利南部一个中型城市,代表了严重的木烟污染,但该地区的室内空气质量知之甚少。2014 年冬季,在特木科市区进行了一项 63 户家庭的现场测量活动,并在此报告。在这项研究中,测量并比较了室内和室外(24 小时)的 PM 及其元素组成。还确定了渗透率参数以及室外/室内对室内 PM 的贡献。还对各种空气质量干预措施和家庭特征如何影响室内 PM 进行了统计评估。本研究确定了室内和室外 PM 的中位数浓度分别为 44.4 和 41.8μg/m。使用硫作为示踪剂,估计了平均渗透率因子(0.62±0.06)。然后,使用简单的质量平衡方法,估计室内和室外对室内 PM 浓度的中位数贡献分别为 12.5 和 26.5μg/m,因此,室内 PM 的 68%来自室外渗透。这一高比例是由于高户外污染和相对较高的家庭空气交换率(中位数:1.06 h)。本研究发现,S、Br 和 Rb 主要来自室外贡献,而 Si、Ca、Ti、Fe 和 As 则来自室内源。使用连续的室内和室外 PM 测量值,在日间期间估计室内源强度的中位数为 75μg PM/min,与文献结果相似。对于傍晚时段,中位数估计值上升到 135μg PM/min,反映了夜间与烹饪和空间加热相关的更强烈的木柴燃烧。(90%置信水平下的)统计测试结果支持智利南部正在进行的柴火炉更换计划(减少排放)和家庭隔热补贴(减少供暖需求),以改善室内空气质量,并表明炉灶改进计划可能也有所帮助。