Li Fajun, Xie Xiaolong, Gao Qian, Tan Liying, Zhou Yanping, Yang Qingbo, Ma Jing, Fu Lan, Tan Hark Hoe, Jagadish Chennupati
Department of Electronic Materials Engineering, Research School of Physics and Engineering, The Australian National University, Canberra 2601, A.C.T., Australia. National Key Laboratory of Tunable Laser Technology, Harbin Institute of Technology, Harbin 150001, People's Republic of China.
Nanotechnology. 2018 Jun 1;29(22):225703. doi: 10.1088/1361-6528/aab009. Epub 2018 Feb 16.
Radiation effects on semiconductor nanowires (NWs) have attracted the attention of the research community due to their potential applications in space and atomic fields. The effective implementation of NW devices in a radiation environment is a matter of concern. Here, the photoluminescence (PL) and time-resolved PL (TRPL) measurements were performed on both GaAs and InP NWs at room temperature before and after 1 MeV H irradiation with fluences ranging from 1 × 10 to 5 × 10 p cm. It is found that the degradation of lifetime is size-dependent, and typically the minority carrier lifetime damage coefficient is closely correlated with the material and NW diameter. Compared to GaAs and InP bulk material counterparts, the lifetime damage coefficient of NWs decreases by a factor of about one order of magnitude. After irradiation, GaAs NWs with a smaller diameter show a much lower lifetime damage coefficient while InP NWs show an increase in carrier radiative lifetime. The increased size-dependent radiation hardness is mainly attributed to the defect sink effect and/or the improvement of a room temperature dynamic annealing mechanism of the NWs. The InP NWs also showed higher radiation tolerance than GaAs NWs.
由于半导体纳米线(NWs)在空间和原子领域的潜在应用,其辐射效应已引起研究界的关注。NW器件在辐射环境中的有效应用是一个值得关注的问题。在此,对GaAs和InP纳米线在室温下进行了1 MeV H辐照(通量范围为1×10至5×10 p cm)前后的光致发光(PL)和时间分辨光致发光(TRPL)测量。发现寿命的退化与尺寸有关,通常少数载流子寿命损伤系数与材料和NW直径密切相关。与GaAs和InP体材料相比,NWs的寿命损伤系数降低了约一个数量级。辐照后,直径较小的GaAs纳米线显示出低得多的寿命损伤系数,而InP纳米线则显示出载流子辐射寿命增加。尺寸依赖性辐射硬度的增加主要归因于缺陷陷阱效应和/或NWs室温动态退火机制的改善。InP纳米线也显示出比GaAs纳米线更高的辐射耐受性。