National Research Council of Canada , Ottawa , Ontario , Canada , K1A 0R6.
KTH Royal Institute of Technology , Stockholm , 100 44 Sweden.
Nano Lett. 2018 May 9;18(5):3047-3052. doi: 10.1021/acs.nanolett.8b00550. Epub 2018 Apr 5.
We report on the site-selected growth of bright single InAsP quantum dots embedded within InP photonic nanowire waveguides emitting at telecom wavelengths. We demonstrate a dramatic dependence of the emission rate on both the emission wavelength and the nanowire diameter. With an appropriately designed waveguide, tailored to the emission wavelength of the dot, an increase in the count rate by nearly 2 orders of magnitude (0.4 to 35 kcps) is obtained for quantum dots emitting in the telecom O-band, showing high single-photon purity with multiphoton emission probabilities down to 2%. Using emission-wavelength-optimized waveguides, we demonstrate bright, narrow-line-width emission from single InAsP quantum dots with an unprecedented tuning range of 880 to 1550 nm. These results pave the way toward efficient single-photon sources at telecom wavelengths using deterministically grown InAsP/InP nanowire quantum dots.
我们报告了在电信波长发射的嵌入 InP 光子纳米线波导中的亮单 InAsP 量子点的选择生长。我们证明了发射率对发射波长和纳米线直径的强烈依赖关系。通过设计适当的波导,针对量子点的发射波长进行调整,可以使在电信 O 波段发射的量子点的计数率增加近 2 个数量级(0.4 到 35 kcps),表现出高的单光子纯度,多光子发射概率低至 2%。使用发射波长优化的波导,我们实现了单 InAsP 量子点的亮窄线宽发射,其调谐范围前所未有,达到 880 至 1550nm。这些结果为使用确定性生长的 InAsP/InP 纳米线量子点在电信波长下实现高效单光子源铺平了道路。