Research Center for Applied Sciences, Academia Sinica, Taipei, 11529, Taiwan.
Department of Photonics and Institute of Electro-Optical Engineering, National Chiao Tung University, Hsinchu, 30010, Taiwan.
Adv Mater. 2018 May;30(21):e1706918. doi: 10.1002/adma.201706918. Epub 2018 Apr 6.
Given the high demand for miniaturized optoelectronic circuits, plasmonic devices with the capability of generating coherent radiation at deep subwavelength scales have attracted great interest for diverse applications such as nanoantennas, single photon sources, and nanosensors. However, the design of such lasing devices remains a challenging issue because of the long structure requirements for producing strong radiation feedback. Here, a plasmonic laser made by using a nanoscale hyperbolic metamaterial cube, called hyperbolic metacavity, on a multiple quantum-well (MQW), deep-ultraviolet emitter is presented. The specifically designed metacavity merges plasmon resonant modes within the cube and provides a unique resonant radiation feedback to the MQW. This unique plasmon field allows the dipoles of the MQW with various orientations into radiative emission, achieving enhancement of spontaneous emission rate by a factor of 33 and of quantum efficiency by a factor of 2.5, which is beneficial for coherent laser action. The hyperbolic metacavity laser shows a clear clamping of spontaneous emission above the threshold, which demonstrates a near complete radiation coupling of the MQW with the metacavity. This approach shown here can greatly simplify the requirements of plasmonic nanolaser with a long plasmonic structure, and the metacavity effect can be extended to many other material systems.
鉴于对小型化光电电路的巨大需求,能够在深亚波长尺度产生相干辐射的等离子体器件已经在各种应用中引起了极大的兴趣,例如纳米天线、单光子源和纳米传感器。然而,由于产生强辐射反馈的长结构要求,此类激光器件的设计仍然是一个挑战。在这里,提出了一种基于多量子阱(MQW)深紫外发射器的纳米级双曲超材料立方体的等离子体激光器,称为双曲超腔。专门设计的超腔将立方体中的等离子体共振模式融合在一起,并为 MQW 提供独特的共振辐射反馈。这种独特的等离子体场允许 MQW 中具有各种取向的偶极子进入辐射发射,自发辐射率提高了 33 倍,量子效率提高了 2.5 倍,这有利于相干激光作用。双曲超腔激光器在阈值以上显示出自发发射的明显箝位,这表明 MQW 与超腔之间实现了近乎完全的辐射耦合。这里展示的方法可以大大简化具有长等离子体结构的等离子体纳米激光器的要求,并且超腔效应可以扩展到许多其他材料系统。