Hughes Stephen, Richter Marten, Knorr Andreas
Opt Lett. 2018 Apr 15;43(8):1834-1837. doi: 10.1364/OL.43.001834.
We present a quantized pseudomode theory for solving system-level cavity quantum electrodynamics with quantum emitters coupled to plasmonic resonators. Exploiting the Green function response of a silver nanoparticle and an exact solution for the input-output coupling, we study the non-Markovian coupling regimes of multi-mode vacuum Rabi oscillations and coherently pumped multi-photon resonances from the higher lying ladder states of collective plasmon modes. The nonlinear pumping regime also facilitates pronounced population inversion of a single two-level atom through multiphoton resonances dominated by dark plasmons.
我们提出了一种量子化赝模理论,用于求解量子发射体与等离子体谐振器耦合的系统级腔量子电动力学。利用银纳米颗粒的格林函数响应和输入-输出耦合的精确解,我们研究了多模真空拉比振荡的非马尔可夫耦合机制,以及集体等离子体模式较高阶梯态的相干泵浦多光子共振。非线性泵浦机制还通过由暗等离子体主导的多光子共振,促进了单个二能级原子的显著粒子数反转。