School of Electronics and Information Technology, State Key Laboratory of Opto-Electronic Materials & Technologies, Guangdong Province Key Laboratory of Display Materials and Technologies , Sun Yat-sen University , Guangzhou 510275 , People's Republic of China.
ACS Appl Mater Interfaces. 2018 May 16;10(19):16596-16604. doi: 10.1021/acsami.8b02233. Epub 2018 May 2.
We report a facile transfer method to fabricate flexible photodetectors directly on tape, wherein the films formed by different processes were integrated together. The tape-based photodetectors with CdS nanowire (NW) active layers exhibited good performances as those fabricated by conventional processes. The obvious persistent photocurrent in our device was eliminated by introducing a conductive polymer poly(3,4-ethylenedioxythiophene)polystyrene sulfonate (PEDOT:PSS) onto the CdS NW layer. By adjusting the concentration of the PEDOT:PSS aqueous solution, a device with a fast response, ultrashort decay time, and relatively large photocurrent was obtained. The decay times were 11.59 and 6.64 ms for devices using electrodes of silver NWs and gold, respectively. These values are much shorter than the shortest decay times (on the order of hundreds of milliseconds) reported previously.
我们报告了一种简便的转移方法,可将不同工艺形成的薄膜直接集成在柔性基底上,从而在柔性基底上制备出光电探测器。基于 CdS 纳米线(NW)的柔性光电探测器具有与传统工艺制备的器件相当的性能。通过在 CdS NW 层上引入导电聚合物聚(3,4-乙撑二氧噻吩)聚苯乙烯磺酸盐(PEDOT:PSS),消除了我们的器件中明显的持久光电流。通过调整 PEDOT:PSS 水溶液的浓度,获得了具有快速响应、超短衰减时间和相对较大光电流的器件。使用银 NW 和金电极的器件的衰减时间分别为 11.59 和 6.64 ms。这些值远短于以前报道的最短衰减时间(数百毫秒量级)。