Centre de Physique Théorique, École Polytechnique, CNRS, Université Paris-Saclay, 91128 Palaiseau, France.
Collège de France, 11 place Marcelin Berthelot, 75005 Paris, France.
Phys Rev Lett. 2018 Mar 23;120(12):126401. doi: 10.1103/PhysRevLett.120.126401.
We investigate the interplay of spin-orbit coupling (SOC) and electronic correlations in Sr_{2}RuO_{4} using dynamical mean-field theory. We find that SOC does not affect the correlation-induced renormalizations, which validates Hund's metal picture of ruthenates even in the presence of the sizable SOC relevant to these materials. Nonetheless, SOC is found to change significantly the electronic structure at k points where a degeneracy applies in its absence. We explain why these two observations are consistent with one another and calculate the effects of SOC on the correlated electronic structure. The magnitude of these effects is found to depend on the energy of the quasiparticle state under consideration, leading us to introduce the notion of an energy-dependent quasiparticle spin-orbit coupling λ^{*}(ω). This notion is generally applicable to all materials in which both the spin-orbit coupling and electronic correlations are sizable.
我们使用动态平均场理论研究了 Sr_{2}RuO_{4} 中自旋轨道耦合(SOC)和电子相关的相互作用。我们发现 SOC 不会影响相关诱导的重整化,这验证了即使在与这些材料相关的可观 SOC 存在的情况下,钌酸盐的 Hund 金属图像也是有效的。然而,SOC 被发现会显著改变在没有 SOC 时处于简并的 k 点处的电子结构。我们解释了为什么这两个观察结果是一致的,并计算了 SOC 对相关电子结构的影响。我们发现这些影响的大小取决于所考虑的准粒子态的能量,这导致我们引入了能量相关准粒子自旋轨道耦合 λ^{*}(ω)的概念。这个概念通常适用于 SOC 和电子相关都很大的所有材料。