School of Civil, Environmental and Architectural Engineering, Korea University, Seoul 136-701, Republic of Korea.
Indian Institute of Technology Guwahati, Guwahati 781039, India.
Ultrason Sonochem. 2018 Jul;45:29-49. doi: 10.1016/j.ultsonch.2018.03.003. Epub 2018 Mar 6.
Heterogeneous sonocatalysis, as an emerging advanced oxidation process (AOP), has shown immense potential in water treatment and been widely demonstrated to remove persistent organic compounds in the past decade. The present article aims to provide a comprehensive review on the development of a heterogeneous catalyst for enhancing the ultrasonic degradation rate of organic pollutants from a viewpoint of sonocatalytic mechanism. The rational design and fundamentals for preparing sonocatalysts are presented in the context of facilitating the heterogeneous nucleation and photo-thermal-catalytic effects as well as considering the mechanical stability and separation capacity of the heterogeneous catalyst. In addition, some new trends, ongoing challenges and possible methods to overcome these challenges are also highlighted and proposed.
多相声催化作为一种新兴的高级氧化工艺(AOP),在水处理方面显示出巨大的潜力,并在过去十年中被广泛证明可去除持久性有机化合物。本文旨在从声催化机制的角度,对用于提高有机污染物超声降解速率的多相催化剂的发展进行全面综述。从促进多相成核和光热催化效应以及考虑多相催化剂的机械稳定性和分离能力的角度,介绍了合理设计和制备声催化剂的基础。此外,还强调并提出了一些新的趋势、当前的挑战以及克服这些挑战的可能方法。