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一种对 Ra、Th、K 和 Cs 的放射性危害特征的建议:空间分布建模。

A suggestion to radiological hazards characterization of Ra, Th, K and Cs: spatial distribution modelling.

机构信息

Kirklareli University, Faculty of Science and Letters, Department of Physics, Campus of Kayali, Kirklareli, Turkey.

Fırat University, Science Faculty, Physics Department, Nuclear Physics Division, TR-23119, Elazig, Turkey.

出版信息

J Hazard Mater. 2018 Jul 5;353:476-489. doi: 10.1016/j.jhazmat.2018.04.042. Epub 2018 Apr 20.

Abstract

Spatial distribution modelling has been proposed to characterize the radiological hazards associated with concentration of natural Ra, Th, K and artificial Cs radionuclides in the nature. These elements have been determined for the sediment samples of the Bafa Lake with the aim of radiation hazard evaluation via a high purity germanium detector gamma spectrometry. Their activity concentrations in sediments are in the ranges of 29.87 ± 2.2-72.56 ± 11 Bq kg dry weight (dw), 31.57 ± 3.5-66.48 ± 8.3 Bq kg (dw), 332.01 ± 12-1092.37 ± 21 and 0.65 ± 0.04-3.96 ± 0.78 Bq kg (dw), respectively. In order to determine the radiological hazard associated with the radioactivity in the samples, the external terrestrial gamma dose rate in air, annual effective dose rate, the radium equivalent activity and the external hazard index are calculated and compared with the data from literature. Moreover, the spatial modelling distributions are obtained visually for radiological hazards characterization of these elements, which are very dangerous in terms of radiological and environmental pollution in the nature. These visual distributions give meaningful information for future researches on the migration of radionuclides in the environment.

摘要

空间分布模型已被提出,用于描述与自然 Ra、Th、K 和人工 Cs 放射性核素浓度相关的辐射危害。通过高纯锗探测器伽马能谱法,对巴法湖的沉积物样本进行了这些元素的测定,目的是进行辐射危害评估。它们在沉积物中的活度浓度范围分别为 29.87±2.2-72.56±11 Bq kg 干重 (dw)、31.57±3.5-66.48±8.3 Bq kg (dw)、332.01±12-1092.37±21 和 0.65±0.04-3.96±0.78 Bq kg (dw)。为了确定与样品放射性相关的辐射危害,计算了空气中的外照射地面伽马剂量率、年有效剂量率、镭当量活度和外照射指数,并与文献数据进行了比较。此外,还对这些元素的辐射危害进行了直观的空间分布模型分析,这些元素在自然的放射性和环境污染方面非常危险。这些直观的分布为未来环境中放射性核素迁移的研究提供了有意义的信息。

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