Department of Materials, ETH Zürich, Switzerland.
Soft Matter. 2018 Jun 6;14(22):4569-4576. doi: 10.1039/c8sm00166a.
Recent experiments have shown that surface stresses in soft materials can have a significant strain-dependence. Here we explore the implications of this surface elasticity to show how, and when, we expect it to arise. We develop the appropriate boundary condition, showing that it simplifies significantly in certain cases. We show that surface elasticity's main role is to stiffen a solid surface's response to in-plane tractions, in particular at length-scales smaller than a characteristic elastocapillary length. We also investigate how surface elasticity affects the Green's-function problem of a line force on a flat, incompressible, linear-elastic substrate. There are significant changes to this solution, especially in that the well-known displacement singularity is regularised. This raises interesting implications for soft phenomena like wetting contact lines, adhesion and friction. Finally, we discuss open questions, future directions, and close ties with existing fields of research.
最近的实验表明,软物质中的表面应力具有显著的应变依赖性。在这里,我们探讨了这种表面弹性的含义,以说明何时以及为何会出现这种情况。我们开发了适当的边界条件,表明在某些情况下它会显著简化。我们表明,表面弹性的主要作用是增强固体表面对平面牵引力的响应,特别是在小于特征弹性毛细长度的长度尺度上。我们还研究了表面弹性如何影响平面、不可压缩、线性弹性衬底上线力的格林函数问题。这个解有显著的变化,特别是众所周知的位移奇点被正则化了。这对诸如润湿接触线、粘附和摩擦等软物质现象产生了有趣的影响。最后,我们讨论了未解决的问题、未来的方向以及与现有研究领域的紧密联系。