Zhang Qian-Hu, Gao Bing, Huang Wei, Yan Xiao-Mei, Cui Sheng-Hui
Key Laboratory of Urban Environment and Health, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China.
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China.
Huan Jing Ke Xue. 2017 Sep 8;38(9):3610-3619. doi: 10.13227/j.hjkx.201702182.
The impacts of reactive nitrogen (Nr) on the environment significantly increase with population and rapid urbanization. In order to study gaseous Nr and Nr loads to waterbodies at the provincial scale, we established anthropogenic emission inventories in prefecture-level cities in Fujian Province and analyzed the changes in Nr emissions for the years 2000, 2005, and 2010. The total Nr emissions were calculated as 538.4, 587.0, and 620.0 Gg in those three years, respectively. The emissions of Nr increased in nine prefecture-level cities except in Zhangzhou. Among these nine cities, Putian is the fastest growing one. The largest emitters were Zhangzhou and Quanzhou, while Ningde and Xiamen were the smallest ones. Agricultural ecosystems and livestock were the main sources of Nr emissions, both of them accounting for more than 90% of total anthropogenic Nr emissions. Despite rapid growth, energy activities had a minor contribution to total Nr emissions. The per area Nr emissions of each prefecture-level city were highest in Xiamen in the southeast coastal area and lowest in Sanming located in the northwest inland region in 2010. However, the patterns of GDP, population, and emission intensities showed the opposite trends to per area Nr emissions, lowest in Xiamen and highest in Nanping. We further discussed the significance of Nr emissions reductions in different areas based on the analysis of the characteristics of Nr emission sources in prefecture-level cities. The results provide a scientific basis for reducing Nr emissions in Fujian Province and its prefecture-level cities.
活性氮(Nr)对环境的影响随着人口增长和快速城市化而显著增加。为了研究省级尺度上气态Nr和水体中Nr负荷,我们建立了福建省地级市的人为排放清单,并分析了2000年、2005年和2010年Nr排放的变化。这三年的Nr排放总量分别计算为538.4、587.0和620.0Gg。除漳州外,九个地级市的Nr排放量都有所增加。在这九个城市中,莆田增长最快。排放最多的是漳州和泉州,而宁德和厦门最少。农业生态系统和畜牧业是Nr排放的主要来源,两者占人为Nr排放总量的90%以上。尽管能源活动迅速增长,但对Nr排放总量的贡献较小。2010年,东南沿海地区的厦门每个地级市的单位面积Nr排放量最高,而位于西北内陆地区的三明最低。然而,GDP、人口和排放强度的模式与单位面积Nr排放量呈现相反趋势,厦门最低,南平最高。基于对地级市Nr排放源特征的分析,我们进一步讨论了不同地区减少Nr排放的意义。研究结果为福建省及其地级市减少Nr排放提供了科学依据。