Department of Civil, Environmental, and Construction Engineering , University of Central Florida , Orlando , Florida , United States.
National High Magnetic Field Laboratory , Florida State University , Tallahassee , Florida , United States.
Environ Sci Technol. 2018 Aug 21;52(16):9380-9390. doi: 10.1021/acs.est.8b01788. Epub 2018 Aug 3.
Eutrophication has been a long-term issue in aquatic environments, where dissolved organic nitrogen (DON) recalcitrance is important. Bioavailable nitrogen qualification and quantification for effluents from stormwater and wastewater are always a challenge. The information in this study deepens the understanding of the interactions between carbon addition and DON decomposition through linear-ditch best management practices for stormwater and groundwater cotreatment. By running a laboratory-scale column study for nitrogen removal using green sorption media, the variation in composition and concentration of DON can be further linked to the population dynamics of microbial species that dominate the nitrification and denitrification processes. With the varying levels of influent total nitrogen concentration, the efficacy of nitrogen removal via biosorption activated media may be realized at the molecular level with ultrahigh resolution Fourier transform ion cyclotron resonance mass spectrometry.
富营养化一直是水生环境中的一个长期问题,其中溶解有机氮(DON)的顽固性是很重要的。对于雨水和废水的排放中的生物可用氮的定性和定量分析一直是一个挑战。本研究的信息通过线性沟渠最佳管理实践对雨水和地下水共同处理加深了对碳添加和 DON 分解之间相互作用的理解。通过使用绿色吸附介质进行实验室规模的氮去除柱研究,可以进一步将 DON 组成和浓度的变化与主导硝化和反硝化过程的微生物物种的种群动态联系起来。随着进水总氮浓度的不同,通过生物吸附活性介质去除氮的效果可以通过超高分辨率傅里叶变换离子回旋共振质谱在分子水平上实现。