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由于南海岸空气盆地范围内减少氮氧化物、挥发性有机化合物和氨排放,预计该盆地中颗粒物浓度的变化。

Projected changes in particulate matter concentrations in the South Coast Air Basin due to basin-wide reductions in nitrogen oxides, volatile organic compounds, and ammonia emissions.

机构信息

a Department of Chemistry , Sacramento City College , Sacramento , CA , USA.

b Global Modeling and Assimilation Office , NASA Goddard Space Flight Center , Greenbelt , MD , USA.

出版信息

J Air Waste Manag Assoc. 2019 Feb;69(2):192-208. doi: 10.1080/10962247.2018.1531795. Epub 2018 Dec 6.

Abstract

An ozone abatement strategy for the South Coast Air Basin (SoCAB) has been proposed by the South Coast Air Quality Management District (SCAQMD) and the California Air Resources Board (ARB). The proposed emissions reduction strategy is focused on the reduction of nitrogen oxide (NO) emissions by the year 2030. Two high PM concentration episodes with high ammonium nitrate compositions occurring during September and November 2008 were simulated with the Community Multi-scale Air Quality model (CMAQ). All simulations were made with same meteorological files provided by the SCAQMD to allow them to be more directly compared with their previous modeling studies. Although there was an overall under-prediction bias, the CMAQ simulations were within an overall normalized mean error of 50%; a range that is considered acceptable performance for PM modeling. A range of simulations of these episodes were made to evaluate sensitivity to NO and ammonia emissions inputs for the future year 2030. It was found that the current ozone control strategy will reduce daily average PM concentrations. However, the targeted NO reductions for ozone were not found to be optimal for reducing PM concentrations. Ammonia emission reductions reduced PM and this might be considered as part of a PM control strategy. Implications: The SCAQMD and the ARB have proposed an ozone abatement strategy for the SoCAB that focuses on NO emission reductions. Their strategy will affect both ozone and PM. Two episodes that occurred during September and November 2008 with high PM concentrations and high ammonium nitrate composition were selected for simulation with different levels of nitrogen oxide and ammonia emissions for the future year 2030. It was found that the ozone control strategy will reduce maximum daily average PM concentrations but its effect on PM concentrations is not optimal.

摘要

南海岸空气质量管理区(SCAQMD)和加利福尼亚空气资源委员会(ARB)提出了南海岸空气盆地(SoCAB)的臭氧减排策略。拟议的减排策略侧重于到 2030 年减少氮氧化物(NO)排放。2008 年 9 月和 11 月发生了两次高 PM 浓度事件,其中铵硝酸盐含量高,使用社区多尺度空气质量模型(CMAQ)进行了模拟。所有模拟均使用 SCAQMD 提供的相同气象文件进行,以便更直接地与之前的建模研究进行比较。尽管存在整体低估偏差,但 CMAQ 模拟的整体归一化平均误差在 50%以内;这是 PM 建模可接受的性能范围。对这些事件进行了一系列模拟,以评估对未来 2030 年 NO 和氨排放量的敏感性。结果发现,目前的臭氧控制策略将降低日平均 PM 浓度。然而,针对臭氧的目标 NO 减排量并未发现对降低 PM 浓度最有效。减少氨排放量可降低 PM,这可能被视为 PM 控制策略的一部分。影响:SCAQMD 和 ARB 已为 SoCAB 提出了一项臭氧减排策略,该策略侧重于减少氮氧化物排放。他们的策略将同时影响臭氧和 PM。选择了 2008 年 9 月和 11 月发生的两次 PM 浓度高且铵硝酸盐含量高的事件,使用不同水平的氮氧化物和氨排放量对未来 2030 年进行模拟。结果发现,臭氧控制策略将降低日最大平均 PM 浓度,但对 PM 浓度的影响并非最佳。

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