CAS Key Laboratory of Bio-based Materials Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao, 266101, Shandong, China.
University of Chinese Academy of Sciences, Beijing, 100049, China.
Chem Rec. 2019 Jul;19(7):1272-1282. doi: 10.1002/tcr.201800100. Epub 2018 Oct 9.
The electrochemical reduction of carbon dioxide (CO ) to value-added products obtains great attention and investigation worldwide in recent years. The commercialization of this green process relies on the progress of relating high-performance electrocatalysts and their feasibility with proper reactor design. The microbial electrosynthesis (MES) is an alternative route to reduce CO with electroactive bio-film electrode as catalyst. This review presents the research status and development of cathode catalysts, particularly focusing on the active sites and development tendency, for highly efficient electrochemical reduction CO from personal viewpoint. Some of our results are also presented to exhibit contributions. MES shows a similar process to the typical electrochemical reduction of CO . Their combination is an important trend, and the future research in this field is full of challenges and opportunities.
近年来，将二氧化碳（CO ）电化学还原为有价值的产品引起了全球的广泛关注和研究。该绿色工艺的商业化依赖于相关高性能电催化剂的进展及其与适当反应器设计的可行性。微生物电合成（MES）是一种替代途径，可利用电活性生物膜电极作为催化剂还原 CO 。本综述从个人角度介绍了阴极催化剂的研究现状和发展，特别是重点介绍了高效电化学还原 CO 的活性位点和发展趋势。还介绍了一些我们的研究结果，以展示我们的贡献。MES 表现出与典型 CO 电化学还原类似的过程。它们的结合是一个重要趋势，该领域的未来研究充满了挑战和机遇。
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