Laboratoire de Chimie-Physique, CNRS, Univ. Paris-Sud, Université Paris Saclay, 91405, Orsay, France.
Institut de Chimie des Substances Naturelles, CNRS UPR 2301, Univ. Paris-Sud, Université Paris-Saclay, 1 Av. de la Terrasse, 91198, Gif-sur-Yvette, France.
J Biol Inorg Chem. 2019 Feb;24(1):39-52. doi: 10.1007/s00775-018-1625-x. Epub 2018 Oct 25.
Human neuroglobin (Ngb) is a hexacoordinated globin which binds some small ligands. Its function is still not well-established, even though Ngb seems to be implicated in the protection against neurodegenerative diseases. It has been shown by molecular dynamics and crystallography that ligand binding could occur thanks to a haem sliding mechanism specific to Ngb. In this paper, we studied some regions which could participate in this mechanism. We used UV-visible spectroscopy, CD and NMR to have a look on the protein structure and NMR and stopped-flow to study the ligand binding properties of the proteins. In the haem environment we mutated the distal histidine H64, the alanine A90 which is on the proximal F helix and the phenylalanine F106 which is close to the haem. We showed that both H64V and A90P variants, which affect the haem coordination, seemed to be important to haem and protein secondary structure stabilities whereas F106L mutation did not affect those properties. Then we confirmed that the cyanide binding kinetics were isomer dependent on wild-type Ngb and A90P and F106L variants. H64V Ngb variant had a behavior similar to wild-type Mb or Hb with a loss of the haem kinetic differentiation. Moreover, our results suggested that one haem isomer was more sensitive to A90P and F106L mutations. Those results brought some evidence that the haem sliding mechanism could occur for the cyanide binding and could be haem isomer dependent. The isomer forms may play distinct roles for the potential function of Ngb in vivo.
人神经球蛋白(Ngb)是一种六配位球蛋白,可结合一些小分子配体。尽管 Ngb 似乎与神经退行性疾病的保护有关,但它的功能仍未得到很好的确定。分子动力学和晶体学表明,配体结合可以通过 Ngb 特有的血红素滑动机制发生。在本文中,我们研究了一些可能参与该机制的区域。我们使用紫外可见光谱、CD 和 NMR 观察蛋白质结构,使用 NMR 和停流技术研究蛋白质的配体结合特性。在血红素环境中,我们突变了远端的组氨酸 H64、位于近端 F 螺旋上的丙氨酸 A90 和靠近血红素的苯丙氨酸 F106。我们表明,影响血红素配位的 H64V 和 A90P 变体似乎对血红素和蛋白质二级结构稳定性很重要,而 F106L 突变则不影响这些性质。然后,我们证实氰化物结合动力学对野生型 Ngb 和 A90P 和 F106L 变体是依赖于异构体的。H64V Ngb 变体的行为类似于野生型 Mb 或 Hb,失去了血红素动力学的差异。此外,我们的结果表明,一种血红素异构体对 A90P 和 F106L 突变更为敏感。这些结果提供了一些证据,表明血红素滑动机制可能发生在氰化物结合中,并且可能依赖于血红素异构体。异构体形式可能在 Ngb 体内的潜在功能中发挥不同的作用。