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中国白洋淀沉积物中氮分布及氨氮释放通量的综合分析。

Comprehensive analysis of nitrogen distributions and ammonia nitrogen release fluxes in the sediments of Baiyangdian Lake, China.

机构信息

State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; University of Chinese Academy of Sciences, Beijing 100049, China.

State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China; University of Chinese Academy of Sciences, Beijing 100049, China.

出版信息

J Environ Sci (China). 2019 Feb;76:319-328. doi: 10.1016/j.jes.2018.05.024. Epub 2018 Jun 14.

Abstract

The condition of Baiyangdian Lake (BYDL) will improve as the Xiongan New Area evolves and fulfills its role of easing overcrowding and supporting economic growth. Water and sediment samples from BYDL were analyzed to provide information on nitrogen (N) contamination in BYDL. The mean ammonium N (NH-N), nitrate N, and total N concentrations in the water samples were 0.36, 0.12, and 2.22 mg/L, respectively, and the ranges were 0.003-8.38, 0.06-0.30, and 1.25-10.34 mg/L, respectively. The N concentrations in water gradually increased from the north to the south of BYDL. Sediment at 90% of the sampling sites was in or above the moderately contaminated class (1000-2000 mg/kg) defined in US Environmental Protection Agency total N pollution standards. Positive NH-N fluxes were found for 28 of the 34 sediment core samples, so the potential for NH-N being released from sediment was relatively high. The NH-N fluxes were 5.35-48.76 mg/m/day, and the mean and maximum fluxes were 8.71 and 48.76 mg/m/day, respectively. Benthic organisms will be affected more by NH-N and NH·HO in the surface sediment pore water (mean concentrations 4.93 and 0.13 mg/L, respectively) than by the other forms of N.

摘要

随着雄安新区的发展和发挥缓解过度拥挤和支持经济增长的作用,白洋淀(BYDL)的状况将得到改善。对 BYDL 的水和泥沙样本进行了分析,以提供有关 BYDL 氮污染的信息。水样中铵态氮(NH-N)、硝酸盐氮和总氮的平均浓度分别为 0.36、0.12 和 2.22mg/L,范围分别为 0.003-8.38、0.06-0.30 和 1.25-10.34mg/L。水样中的 N 浓度从北到南逐渐增加。在 90%的采样点,沉积物处于或高于美国环境保护署总氮污染标准定义的中度污染等级(1000-2000mg/kg)。在 34 个沉积物岩芯样本中有 28 个样本发现正的 NH-N 通量,因此沉积物中 NH-N 释放的潜力相对较高。NH-N 通量为 5.35-48.76mg/m/天,平均和最大通量分别为 8.71 和 48.76mg/m/天。底栖生物将受到表层沉积物孔隙水中 NH-N 和 NH·HO(分别为 4.93 和 0.13mg/L)的影响大于其他形式的 N。

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