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[强工业城市岩溶地下水系统中多环芳烃的分布与来源]

[Distribution and Sources of Polycyclic Aromatic Hydrocarbons in a Karst Groundwater System in a Strongly Industrial City].

作者信息

Miao Ying, Kong Xiang-Sheng, Li Cheng-Zhan

机构信息

Key Laboratory of Karst Dynamics, Ministry of Natural Resources & Guangxi, Institute of Karst Geology, Chinese Academy of Geological Sciences, Guilin 541004, China.

出版信息

Huan Jing Ke Xue. 2019 Jan 8;40(1):239-247. doi: 10.13227/j.hjkx.201805212.

Abstract

To understand the spatiotemporal variation characteristics and sources of polycyclic aromatic hydrocarbons in karst groundwater in a strongly industrial city, the authors collected 23 groundwater samples in the water and dry period in Liuzhou using component spectra of 16 types of polycyclic aromatic hydrocarbons in combination with the physical and chemical properties and analyzed the spatiotemporal variation characteristics and sources of the polycyclic aromatic hydrocarbons (PAHs) in karst groundwater in heavy industrial city. The results show that the average concentration of ∑PAHs in the groundwater in the wet period has an order of Liubei District > Liudong District > Liuxi District > Jila Underground River and the concentration proportion of PAHs decreases with the increase of the molecular weight, while the order in the dry period is Jila Underground River > Liubei District > Liuxi District > Liudong District. The PAHs in the groundwater during the dry season have a high pollution level, while a low pollution level is observed in the wet season. The main sources of PAHs are organic matter burns at high temperature such as fossil fuel, which are produced by human activities such as industrial processes, transportation, heating, and cooking.

摘要

为了解某重工业化城市岩溶地下水中多环芳烃的时空变化特征及来源,作者结合16种多环芳烃的组分谱,采集了柳州市丰水期和枯水期的23个地下水样,并分析了该重工业化城市岩溶地下水中多环芳烃(PAHs)的时空变化特征及来源。结果表明,丰水期地下水中∑PAHs平均浓度顺序为柳北区>柳东新区>柳西区>基隆地下河,且PAHs浓度比例随分子量增大而降低;枯水期顺序为基隆地下河>柳北区>柳西区>柳东新区。枯水期地下水中PAHs污染水平较高,而丰水期污染水平较低。PAHs主要来源为化石燃料等高温下的有机物燃烧,由工业生产、交通运输、取暖和烹饪等人类活动产生。

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