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铜氧化物高温超导体中量子临界点的热力学特征。

Thermodynamic signatures of quantum criticality in cuprate superconductors.

机构信息

Institut Néel, Université Grenoble Alpes, Grenoble, France.

Institut quantique, Département de physique and RQMP, Université de Sherbrooke, Sherbrooke, Québec, Canada.

出版信息

Nature. 2019 Mar;567(7747):218-222. doi: 10.1038/s41586-019-0932-x. Epub 2019 Feb 13.

Abstract

The three central phenomena of cuprate (copper oxide) superconductors are linked by a common doping level p*-at which the enigmatic pseudogap phase ends and the resistivity exhibits an anomalous linear dependence on temperature, and around which the superconducting phase forms a dome-shaped area in the phase diagram. However, the fundamental nature of p* remains unclear, in particular regarding whether it marks a true quantum phase transition. Here we measure the specific heat C of the cuprates Eu-LSCO and Nd-LSCO at low temperature in magnetic fields large enough to suppress superconductivity, over a wide doping range that includes p*. As a function of doping, we find that C/T is strongly peaked at p* (where C is the electronic contribution to C) and exhibits a log(1/T) dependence as temperature T tends to zero. These are the classic thermodynamic signatures of a quantum critical point, as observed in heavy-fermion and iron-based superconductors at the point where their antiferromagnetic phase comes to an end. We conclude that the pseudogap phase of cuprates ends at a quantum critical point, the associated fluctuations of which are probably involved in d-wave pairing and the anomalous scattering of charge carriers.

摘要

铜氧化物(氧化铜)超导体的三个中心现象通过一个共同的掺杂水平 p* 联系在一起,在这个掺杂水平上,神秘的赝能隙相结束,电阻率表现出异常的线性温度依赖性,而超导相在相图中形成一个圆顶形区域。然而,p* 的基本性质仍不清楚,特别是它是否标志着一个真正的量子相变。在这里,我们在足以抑制超导性的磁场中,在包括 p* 在内的宽掺杂范围内,测量了铜酸盐 Eu-LSCO 和 Nd-LSCO 的低温比热 C。作为掺杂的函数,我们发现 C/T 在 p* 处强烈峰值(其中 C 是 C 的电子贡献),并且随着温度 T 趋于零,表现出 log(1/T) 的依赖性。这些是量子临界点的经典热力学特征,如在重费米子和铁基超导体中观察到的那样,在那里它们的反铁磁相结束。我们得出结论,铜酸盐的赝能隙相在量子临界点结束,与该临界点相关的涨落可能与 d 波配对和电荷载流子的异常散射有关。

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