Institut Néel, Université Grenoble Alpes, Grenoble, France.
Institut quantique, Département de physique and RQMP, Université de Sherbrooke, Sherbrooke, Québec, Canada.
Nature. 2019 Mar;567(7747):218-222. doi: 10.1038/s41586-019-0932-x. Epub 2019 Feb 13.
The three central phenomena of cuprate (copper oxide) superconductors are linked by a common doping level p*-at which the enigmatic pseudogap phase ends and the resistivity exhibits an anomalous linear dependence on temperature, and around which the superconducting phase forms a dome-shaped area in the phase diagram. However, the fundamental nature of p* remains unclear, in particular regarding whether it marks a true quantum phase transition. Here we measure the specific heat C of the cuprates Eu-LSCO and Nd-LSCO at low temperature in magnetic fields large enough to suppress superconductivity, over a wide doping range that includes p*. As a function of doping, we find that C/T is strongly peaked at p* (where C is the electronic contribution to C) and exhibits a log(1/T) dependence as temperature T tends to zero. These are the classic thermodynamic signatures of a quantum critical point, as observed in heavy-fermion and iron-based superconductors at the point where their antiferromagnetic phase comes to an end. We conclude that the pseudogap phase of cuprates ends at a quantum critical point, the associated fluctuations of which are probably involved in d-wave pairing and the anomalous scattering of charge carriers.
铜氧化物(氧化铜)超导体的三个中心现象通过一个共同的掺杂水平 p* 联系在一起,在这个掺杂水平上,神秘的赝能隙相结束,电阻率表现出异常的线性温度依赖性,而超导相在相图中形成一个圆顶形区域。然而,p* 的基本性质仍不清楚,特别是它是否标志着一个真正的量子相变。在这里,我们在足以抑制超导性的磁场中,在包括 p* 在内的宽掺杂范围内,测量了铜酸盐 Eu-LSCO 和 Nd-LSCO 的低温比热 C。作为掺杂的函数,我们发现 C/T 在 p* 处强烈峰值(其中 C 是 C 的电子贡献),并且随着温度 T 趋于零,表现出 log(1/T) 的依赖性。这些是量子临界点的经典热力学特征,如在重费米子和铁基超导体中观察到的那样,在那里它们的反铁磁相结束。我们得出结论,铜酸盐的赝能隙相在量子临界点结束,与该临界点相关的涨落可能与 d 波配对和电荷载流子的异常散射有关。