Center for Nanophysics and Advanced Materials and Department of Physics, University of Maryland, College Park, MD 20742, USA.
Proc Natl Acad Sci U S A. 2012 May 29;109(22):8440-4. doi: 10.1073/pnas.1120273109. Epub 2012 May 9.
In the high-temperature cuprate superconductors, the pervasiveness of anomalous electronic transport properties suggests that violation of conventional Fermi liquid behavior is closely tied to superconductivity. In other classes of unconventional superconductors, atypical transport is well correlated with proximity to a quantum critical point, but the relative importance of quantum criticality in the cuprates remains uncertain. Here, we identify quantum critical scaling in the electron-doped cuprate material La(2-x)Ce(x)CuO(4) with a line of quantum critical points that surrounds the superconducting phase as a function of magnetic field and charge doping. This zero-temperature phase boundary, which delineates a metallic Fermi liquid regime from an extended non-Fermi liquid ground state, closely follows the upper critical field of the overdoped superconducting phase and gives rise to an expanse of distinct non-Fermi liquid behavior at finite temperatures. Together with signatures of two distinct flavors of quantum fluctuations, these facts suggest that quantum criticality plays a significant role in shaping the anomalous properties of the cuprate phase diagram.
在高温铜酸盐超导体中,反常电子输运性质的普遍性表明,违反传统费米液体行为与超导性密切相关。在其他非常规超导体类别中,非典型输运与接近量子临界点密切相关,但在铜酸盐中量子临界点的相对重要性仍不确定。在这里,我们在电子掺杂铜酸盐材料 La(2-x)Ce(x)CuO(4)中识别出量子临界缩放,该材料具有一系列量子临界点,这些临界点作为磁场和电荷掺杂的函数围绕超导相。这条零温相边界将金属费米液体区域与扩展的非费米液体基态区分开来,它与过掺杂超导相的上临界场密切相关,并在有限温度下产生广泛的独特非费米液体行为。与两种不同量子涨落特征一起,这些事实表明量子临界点在塑造铜酸盐相图的异常性质方面起着重要作用。