Kim Nayoung, Park Hyungmin, Do Hyungrok
Langmuir. 2019 Mar 5;35(9):3308-3318. doi: 10.1021/acs.langmuir.8b04083. Epub 2019 Feb 21.
As an example of photon-matter interaction, we experimentally investigate the temporal evolution of a millimeter-sized cavitation bubble, induced by focusing a continuous-wave laser on a metallic plate in tap water. Our major interests are to understand the mechanism of bubble growth/shrinkage for a long time duration up to O(10) seconds and to draw the time-dependency relation of a bubble size, depending on the incident laser power. With the time passed after the laser with different power is focused, it is found that the phase change and/or transport of dissolved gas into the bubble play a dominant role in determining the bubble growth and shrinkage. Thus, we propose two stages in terms of time and three regimes depending on the incident energy, in which the evolutions of cavitation bubble in short and long time durations are distinctively identified. In regime I (lower incident power), the water nearby the focal point undergoes a phase change, resulting in an initial rapid growth of a bubble (first stage), but the convection flow due to locally heated surface causes the bubble to shrink at later times (second stage). As the laser power increases (regime III), more dissolved gas in the surrounding water enters the growing bubble and prevents the water phase from being absorbed into the bubble. Thus, the bubble growth is dominated by the dissolved gas. Between regimes I and III, there is a transitional regime II in which both the phase change of water and the dissolved gas contribute to the bubble evolution. We further our understandings by developing the relations about the time-dependency of bubble size for each stage and regime, which agree well with the measured data. The scaling relations are also validated with different conditions of liquid such as degassed water and NaCl solution. While previous studies have mostly focused on the nano- and/or microsized bubble generation in a very short time (less than 1 s), we think that the present results will extend our knowledge on how to predict and control the size of laser-induced cavitation bubble for longer time duration.
作为光子与物质相互作用的一个例子,我们通过将连续波激光聚焦在自来水中的金属板上,对毫米级空化气泡的时间演化进行了实验研究。我们主要感兴趣的是了解长达O(10)秒的长时间内气泡生长/收缩的机制,并绘制气泡尺寸与入射激光功率的时间依赖关系。在聚焦不同功率的激光后随着时间的推移,发现溶解气体的相变和/或向气泡中的传输在决定气泡的生长和收缩中起主导作用。因此,我们根据时间提出了两个阶段,并根据入射能量提出了三种状态,其中空化气泡在短时间和长时间内的演化被明确区分。在状态I(较低的入射功率)下,焦点附近的水发生相变,导致气泡初始快速生长(第一阶段),但由于局部加热表面引起的对流使气泡在后期收缩(第二阶段)。随着激光功率增加(状态III),周围水中更多的溶解气体进入正在生长的气泡,并阻止水相被吸收到气泡中。因此,气泡的生长由溶解气体主导。在状态I和III之间,存在一个过渡状态II,其中水的相变和溶解气体都对气泡的演化有贡献。我们通过建立每个阶段和状态下气泡尺寸的时间依赖关系来进一步加深理解,这些关系与测量数据吻合良好。这些标度关系也在不同液体条件下(如脱气水和NaCl溶液)得到了验证。虽然以前的研究大多集中在极短时间(小于1秒)内纳米级和/或微米级气泡的产生,但我们认为目前的结果将扩展我们关于如何在更长时间内预测和控制激光诱导空化气泡尺寸的知识。