Department of Chemistry, UiT - The Arctic University of Norway, 9037 Tromsø, Norway.
Org Biomol Chem. 2019 Mar 20;17(12):3159-3166. doi: 10.1039/c9ob00168a.
Free-base meso-triarylcorroles have been found to undergo oxidative coupling with an excess of pyrrole in dichloromethane in the presence of 2,3-dichloro-5,6-dicyano-1,4-benzoquinone (DDQ) affording 5/10-pyrrole-appended isocorroles in reasonable yields (35-60%) and in a matter of seconds. The free-base isocorrole ligands could all be complexed to copper with Cu(OAc)2·H2O in chloroform/methanol in 55-80% yields. Single-crystal X-ray structures of two of the new compounds (H2[5-pyr-TpOMePiC] and Cu[10-pyr-TpOMePiC]) revealed planar macrocycles with rms atomic displacements of only 0.02 and 0.06 Å relative to their respective best-fit C19N4 planes. Both free-base and Cu(ii)-complexed isocorroles exhibit richly featured UV-vis-NIR spectra with red/NIR absorption maxima at ∼650 nm and ∼725 nm for the free-bases and ∼800-850 nm for the copper complexes, suggesting potential applications in photodynamic therapy. Cyclic voltammetric analyses of five of the Cu complexes revealed fully reversible redox cycles with multiple oxidation and reduction features.
游离碱meso-三芳基corrole 在二氯甲烷中与过量吡咯在 2,3-二氯-5,6-二氰基-1,4-苯醌(DDQ)存在下发生氧化偶联,以合理的产率(35-60%)和几秒钟的时间得到 5/10-吡咯取代的同二corrole。游离碱同二 corrole 配体都可以与 Cu(OAc)2·H2O 在氯仿/甲醇中以 55-80%的产率络合到铜上。两个新化合物(H2[5-pyr-TpOMePiC]和 Cu[10-pyr-TpOMePiC])的单晶 X 射线结构显示出平面大环,其相对各自最佳拟合的 C19N4 平面的均方根原子位移仅为 0.02 和 0.06 Å。游离碱和 Cu(ii)-配合的同二 corrole 都表现出丰富的紫外可见近红外光谱,游离碱的最大吸收波长在 ∼650 nm 和 ∼725 nm,铜配合物的最大吸收波长在 ∼800-850 nm,这表明它们在光动力治疗中有潜在的应用。五种 Cu 配合物的循环伏安分析显示出完全可逆的氧化还原循环,具有多个氧化和还原特征。