Ma Churong, Yan Jiahao, Huang Yingcong, Yang Guowei
State Key Laboratory of Optoelectronic Materials and Technologies, Nanotechnology Research Center, School of Materials Science & Engineering, Sun Yat-sen University, Guangdong, Guangzhou, 510275, P. R. China.
Small. 2019 May;15(18):e1900546. doi: 10.1002/smll.201900546. Epub 2019 Apr 8.
Fano resonance has been observed in a wide variety of nanophotonic structures such as photonic crystals, plasmonic structures, and metamaterials. It arises from the interference of discrete resonance states with broadband continuum states. As an emerging nanophotonic material, high-index all-dielectric nanomaterials provide a new platform to achieve Fano resonance by virtue of the simultaneous excited electric and magnetic resonances. However, to date, Fano resonance in the visible region has not been observed in individual high-index all-dielectric nanoparticles. Here, for the first time, the experimental observation of the directional Fano resonance is reported in an individual GaAs nanospheroid. The special geometry enables GaAs nanospheroids to generate spectrally overlapped electric and magnetic dipole resonances, which enhances their spectral coupling, giving rise to asymmetric-shaped backward scattering spectrum. This directional Fano resonance can be tuned by the aspect ratio of nanospheroids as well as excitation polarization. In addition, efficient directional light scattering is realized at the total scattering peak of the GaAs nanospheroid. The forward-to-backward scattering ratio can be largely enhanced due to Fano dip in the backward scattering spectrum. These findings suggest that high-index all-dielectric nanospheroid is a promising candidate for directional sources and optical switches.
在各种纳米光子结构中都观察到了法诺共振,如光子晶体、等离子体结构和超材料。它源于离散共振态与宽带连续态的干涉。作为一种新兴的纳米光子材料,高折射率全介质纳米材料凭借同时激发的电共振和磁共振,为实现法诺共振提供了一个新平台。然而,迄今为止,在单个高折射率全介质纳米颗粒中尚未观察到可见光区域的法诺共振。在此,首次报道了在单个砷化镓纳米球体中对定向法诺共振的实验观察。这种特殊的几何形状使砷化镓纳米球体能够产生光谱重叠的电偶极子共振和磁偶极子共振,增强了它们的光谱耦合,产生不对称形状的后向散射光谱。这种定向法诺共振可以通过纳米球体的纵横比以及激发极化来调节。此外,在砷化镓纳米球体的总散射峰处实现了高效的定向光散射。由于后向散射光谱中的法诺凹陷,前向散射与后向散射之比可大幅提高。这些发现表明,高折射率全介质纳米球体是定向光源和光开关的有前途的候选材料。