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全介质纳米粒子低聚物中的 Fano 共振观察。

Observation of Fano resonances in all-dielectric nanoparticle oligomers.

机构信息

Nonlinear Physics Centre, Research School of Physics and Engineering, The Australian National University, Canberra, ACT, 0200, Australia.

出版信息

Small. 2014 May 28;10(10):1985-90. doi: 10.1002/smll.201303612. Epub 2014 Feb 25.

Abstract

It is well-known that oligomers made of metallic nanoparticles are able to support sharp Fano resonances originating from the interference of two plasmonic resonant modes with different spectral width. While such plasmonic oligomers suffer from high dissipative losses, a new route for achieving Fano resonances in nanoparticle oligomers has opened up after the recent experimental observations of electric and magnetic resonances in low-loss dielectric nanoparticles. Here, light scattering by all-dielectric oligomers composed of silicon nanoparticles is studied experimentally for the first time. Pronounced Fano resonances are observed for a variety of lithographically-fabricated heptamer nanostructures consisting of a central particle of varying size, encircled by six nanoparticles of constant size. Based on a full collective mode analysis, the origin of the observed Fano resonances is revealed as a result of interference of the optically-induced magnetic dipole mode of the central particle with the collective mode of the nanoparticle structure. This allows for effective tuning of the Fano resonance to a desired spectral position by a controlled size variation of the central particle. Such optically-induced magnetic Fano resonances in all-dielectric oligomers offer new opportunities for sensing and nonlinear applications.

摘要

众所周知,由金属纳米粒子组成的低聚物能够支持源于两种具有不同光谱宽度的等离子体共振模式干涉的尖锐的 Fano 共振。虽然这种等离子体低聚物存在高耗散损耗,但在最近观察到低损耗介电纳米粒子中的电和磁共振之后,为在纳米粒子低聚物中实现 Fano 共振开辟了一条新途径。在这里,首次对由硅纳米粒子组成的全介电低聚物的光散射进行了实验研究。对于各种由光刻制造的七聚体纳米结构,观察到了明显的 Fano 共振,这些结构由一个大小不断变化的中心粒子和六个大小不变的纳米粒子环绕而成。基于全集体模式分析,揭示了观察到的 Fano 共振的起源,这是由于中心粒子的光诱导磁偶极模式与纳米粒子结构的集体模式之间的干涉。这使得通过对中心粒子的受控尺寸变化,可以将 Fano 共振有效地调谐到所需的光谱位置。全介电低聚物中的这种光诱导磁 Fano 共振为传感和非线性应用提供了新的机会。

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