Grasset Romain, Gallais Yann, Sacuto Alain, Cazayous Maximilien, Mañas-Valero Samuel, Coronado Eugenio, Méasson Marie-Aude
Laboratoire Matériaux et Phénomènes Quantiques, Université Paris Diderot, Sorbonne Paris Cité, UMR No. 7162, CNRS, 75013 Paris, France.
Universidad de Valencia (ICMol), Catedratico José Beltran Martinez, 46980 Paterna, Spain.
Phys Rev Lett. 2019 Mar 29;122(12):127001. doi: 10.1103/PhysRevLett.122.127001.
The pressure evolution of the Raman active electronic excitations of the transition metal dichalcogenides 2H-TaS_{2} is followed through the pressure phase diagram embedding incommensurate charge-density-wave and superconducting states. At high pressure, the charge-density wave is found to collapse at 8.5 GPa. In the coexisting charge-density-wave and superconducting orders, we unravel a strong in-gap superconducting mode, attributed to a Higgs mode, coexisting with the expected incoherent Cooper-pair breaking signature. The latter remains in the pure superconducting state reached above 8.5 GPa. Our report constitutes a new observation of such Raman active Higgs mode since the long-standing unique case 2H-NbSe_{2}.
通过包含非公度电荷密度波和超导态的压力相图,跟踪过渡金属二硫属化物2H-TaS₂的拉曼活性电子激发的压力演变。在高压下,发现电荷密度波在8.5吉帕斯卡时崩塌。在共存的电荷密度波和超导序中,我们揭示了一种强带隙超导模式,归因于希格斯模式,它与预期的非相干库珀对破坏特征共存。后者保留在8.5吉帕斯卡以上达到的纯超导态中。自长期以来独一无二的2H-NbSe₂案例以来,我们的报告构成了对这种拉曼活性希格斯模式的新观察。