Chen Zhiquan, Li Ping, Zhang Shi, Chen Yiqin, Liu Peng, Duan Huigao
State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body, College of Mechanical and Vehicle Engineering, Hunan University, Changsha 410082, People's Republic of China. College of Information and Electronic Engineering, Hunan City University, Yiyang 413000, People's Republic of China.
Nanotechnology. 2019 Aug 16;30(33):335201. doi: 10.1088/1361-6528/ab1b89. Epub 2019 Apr 23.
The phenomenon of extraordinary optical transmission (EOT) caused by light through metallic nanohole arrays has attracted significant attention due to its potential applications for monolithic color filters and ultrasensitive label-free biosensing. However, the EOT spectra of these nanohole arrays have multiple resonance peaks that are spectrally close to each other due to the multiple resonance modes generated by different media on the upper and lower surfaces of metal. In addition, owing to the absorption loss of metal and the scattering of holes, the EOT resonance peaks have low transmission coefficient for practical applications. In this work, utilizing a tapered nanohole arrays structure which is stacked by multiple cylindrical holes with the same depth but different radii, we show that tapered nanohole arrays can effectively suppress the excitation of multiple resonance peaks, and a single EOT peak emerges in the transmission spectrum and simultaneously exhibits significantly enhanced transmission (∼7 times) and narrow linewidth (∼15 nm). The enhanced EOT of tapered nanohole arrays can be also found in other wavelength regions and plasmonic materials. Benefiting from isolated transmission peak, high transmission efficiency and extremely narrow linewidth, a highly sensitive plasmonic nanosensor with sensitivity of 1580 nm/RIU and figure of merit of 105 can be attained. We believe that the tapered nanohole structure would enable applications for ultrasensitive sensors, switches and efficient filters.
由光穿过金属纳米孔阵列所引起的超常光学透射(EOT)现象,因其在单片式彩色滤光片和超灵敏无标记生物传感方面的潜在应用而备受关注。然而,这些纳米孔阵列的EOT光谱具有多个共振峰,由于金属上下表面不同介质产生的多种共振模式,这些共振峰在光谱上彼此接近。此外,由于金属的吸收损耗和孔的散射,EOT共振峰在实际应用中的透射系数较低。在这项工作中,我们利用一种由多个深度相同但半径不同的圆柱形孔堆叠而成的锥形纳米孔阵列结构,表明锥形纳米孔阵列能够有效抑制多个共振峰的激发,并且在透射光谱中出现单个EOT峰,同时呈现出显著增强的透射率(约7倍)和窄线宽(约15 nm)。锥形纳米孔阵列增强的EOT在其他波长区域和等离子体材料中也能被发现。受益于孤立的透射峰、高传输效率和极窄的线宽,可实现灵敏度为1580 nm/RIU且品质因数为105的高灵敏度等离子体纳米传感器。我们相信,锥形纳米孔结构将能够应用于超灵敏传感器、开关和高效滤波器。