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真空干燥处理的具有高效蓝到绿光电转换功能的微米厚稳定CsPbBr钙钛矿薄膜

Vacuum-Drying Processed Micrometer-Thick Stable CsPbBr Perovskite Films with Efficient Blue-To-Green Photoconversion.

作者信息

Yin Yongming, Ali Muhammad Umair, Liu Ming, Miao Jingsheng, Peng Wenxiang, Li Dongze, Chen Shujhih, Lee Chiayu, Meng Hong

机构信息

School of Advanced Materials, Shenzhen Graduate School, Peking University, Shenzhen, 518055, China.

Shenzhen China Star Optoelectronics Semiconductor Display Technology Co., Ltd. (CSOT), Shenzhen, 518132, China.

出版信息

Small. 2019 Aug;15(31):e1901954. doi: 10.1002/smll.201901954. Epub 2019 Jun 13.

Abstract

Metal halide perovskite materials have attracted great attention owing to their fascinating optoelectronic characteristics and low cost fabrication via facile solution processing. One of the potential applications of these materials is to employ them as color-conversion layers (CCLs) for visible blue light to achieve full-color displays. However, obtaining thick perovskite films to realize complete color conversion is a key challenge. Here, the fabrication of micrometer-level thick CsPbBr perovskite films is presented through a facile vacuum drying approach. An efficient green photoconversion is realized in a 3.8 µm thick film from blue light @ 463 nm. For a back luminance of 1000 cd m , the brightness of the resulting green emission can reach as high as 200 cd m . Furthermore, only ≈2% of decay in brightness is observed when the films are tested after 18 days of exposure to ambient environment. In addition, a potential design is also proposed for full-color displays with perovskite materials incorporated as CCLs.

摘要

金属卤化物钙钛矿材料因其迷人的光电特性以及通过简便的溶液处理实现低成本制造而备受关注。这些材料的潜在应用之一是将它们用作可见蓝光的颜色转换层(CCL)以实现全彩显示。然而,获得厚的钙钛矿薄膜以实现完全的颜色转换是一项关键挑战。在此,通过一种简便的真空干燥方法展示了微米级厚的CsPbBr钙钛矿薄膜的制备。在3.8 µm厚的薄膜中,对于463 nm的蓝光实现了高效的绿色光转换。对于1000 cd m²的背光源亮度,所产生的绿色发射的亮度可高达200 cd m²。此外,当薄膜在暴露于环境环境18天后进行测试时,仅观察到约2%的亮度衰减。此外,还提出了一种将钙钛矿材料用作CCL的全彩显示的潜在设计。

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