Kohler Bern
Department of Chemistry and Biochemistry, The Ohio State University, 100W. 18th Ave., Columbus, OH 43210, USA.
Faraday Discuss. 2019 Jul 11;216(0):564-573. doi: 10.1039/c9fd90030f.
The ability to characterize and control the energy and charge transfer events triggered by the photoexcitation of molecules and materials is of fundamental importance to many fields, including the sustainable capture and conversion of solar energy. This article summarizes the papers that were presented and discussed at the recent Faraday discussion meeting on ultrafast photoinduced energy and charge transfer. Ultrafast laser spectroscopy and theory were at the center of discussions on photoinduced phenomena in biological and nanoscale systems of interacting absorbers. Many of the questions that motivate this field of science have occupied scientists for many decades, as a look back to a Faraday discussion meeting that took place 60 years earlier reveals.
表征和控制由分子和材料的光激发引发的能量和电荷转移事件的能力,对包括太阳能的可持续捕获和转换在内的许多领域至关重要。本文总结了在最近关于超快光致能量和电荷转移的法拉第讨论会上发表和讨论的论文。超快激光光谱学和理论是生物和纳米级相互作用吸收体系统中光致现象讨论的核心。正如回顾60年前举行的一次法拉第讨论会所揭示的那样,推动这一科学领域发展的许多问题已经困扰科学家数十年了。