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异质结构石墨相氮化碳的光催化应用:污染物降解、制氢(水分解)及一氧化碳还原

Photocatalytic Applications of Heterostructure Graphitic Carbon Nitride: Pollutant Degradation, Hydrogen Gas Production (water splitting), and CO Reduction.

作者信息

Darkwah Williams Kweku, Oswald Kivyiro Adinas

机构信息

Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, 1 Xikang Road, Nanjing, 210098, People's Republic of China.

Department of Biochemistry, School of Biological Sciences, University of Cape Coast, Cape Coast, Ghana.

出版信息

Nanoscale Res Lett. 2019 Jul 12;14(1):234. doi: 10.1186/s11671-019-3070-3.

DOI:10.1186/s11671-019-3070-3
PMID:31300944
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6626089/
Abstract

Fabrication of the heterojunction composites photocatalyst has attained much attention for solar energy conversion due to their high optimization of reduction-oxidation potential as a result of effective separation of photogenerated electrons-holes pairs. In this review, the background of photocatalysis, mechanism of photocatalysis, and the several researches on the heterostructure graphitic carbon nitride (g-CN) semiconductor are discussed. The advantages of the heterostructure g-CN over their precursors are also discussed. The conclusion and future perspectives on this emerging research direction are given. This paper gives a useful knowledge on the heterostructure g-CN and their photocatalytic mechanisms and applications. IMPACT STATEMENTS: The paper on g-C3N4 Nano-based photocatalysts is expected to enlighten scientists on precise management and evaluating the environment, which may merit prospect research into developing suitable mechanism for energy, wastewater treatment and environmental purification.

摘要

异质结复合光催化剂的制备因其能有效分离光生电子-空穴对,高度优化还原-氧化电位,在太阳能转换方面备受关注。在本综述中,讨论了光催化的背景、光催化机理以及对异质结构石墨相氮化碳(g-CN)半导体的若干研究。还讨论了异质结构g-CN相对于其前驱体的优势。给出了关于这一新兴研究方向的结论和未来展望。本文提供了关于异质结构g-CN及其光催化机理和应用的有用知识。影响声明:关于基于g-C3N4纳米的光催化剂的论文有望启发科学家精确管理和评估环境,这可能值得对开发适合能源、废水处理和环境净化的机制进行前瞻性研究。

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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b344/6626089/164d3409b1b9/11671_2019_3070_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b344/6626089/b6385fd2ecd4/11671_2019_3070_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b344/6626089/e0b7630e52d5/11671_2019_3070_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b344/6626089/7f88f8fed7dc/11671_2019_3070_Fig8_HTML.jpg
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