Tianjin Key Laboratory of Indoor Air Environmental Quality Control, School of Environmental Science and Engineering, Tianjin University, 92 Weijin Road, Nankai District, Tianjin 300072, China; Key Laboratory of Efficient Utilization of Low and Medium Grade Energy (Tianjin University), Ministry of Education, Tianjin 300072, China.
Tianjin Key Laboratory of Indoor Air Environmental Quality Control, School of Environmental Science and Engineering, Tianjin University, 92 Weijin Road, Nankai District, Tianjin 300072, China.
Bioresour Technol. 2019 Oct;290:121781. doi: 10.1016/j.biortech.2019.121781. Epub 2019 Jul 10.
As one of the most mature carbon capture technologies, thermal regeneration of rich CO absorption solvent is a crucial challenge due to its high energy consumption (typically in the range of 3-6 MJ/kg CO). In this work, a concept of bio-regeneration was proposed using microalgae to convert bicarbonate (which is one of the dominant components in rich solution) into value-added biomass. To evaluate the performance of bio-regeneration, different rich solution (including NHHCO, KHCO and NaHCO) were investigated. Experimental results indicated that NHHCO could be a promising bicarbonate carrier for the proposed absorption-microalgae hybrid process, which had a higher biomass productivity (55.36 mg·L·d) compared to KHCO and NaHCO and carbon sequestration capacity could be up to 158.3 mg·L·d. Meanwhile, pH adjustment was an effective approach to further intensify the performance of hybrid process. As a result, bio-regeneration of solvents could be a promising alternative to the conventional thermal regeneration.
作为最成熟的碳捕集技术之一,富 CO 吸收溶剂的热再生由于其高能耗(通常在 3-6MJ/kgCO 范围内)而成为一个关键挑战。在这项工作中,提出了一种使用微藻进行生物再生的概念,将碳酸氢盐(富液中的主要成分之一)转化为增值生物质。为了评估生物再生的性能,研究了不同的富液(包括 NHHCO、KHCO 和 NaHCO)。实验结果表明,NHHCO 可以作为所提出的吸收-微藻混合工艺的有前途的碳酸氢盐载体,与 KHCO 和 NaHCO 相比,其生物质生产率更高(55.36mg·L·d),碳捕集能力可达 158.3mg·L·d。同时,pH 调节是进一步强化混合工艺性能的有效方法。因此,溶剂的生物再生可能是传统热再生的一种有前途的替代方法。