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CeNi(AsP)中稀载流子极限下的重费米子量子临界性。

Heavy fermion quantum criticality at dilute carrier limit in CeNi(AsP).

作者信息

Chen Jian, Wang Zhen, Li Yupeng, Feng Chunmu, Dai Jianhui, Xu Zhu'an, Si Qimiao

机构信息

Zhejiang Province Key Laboratory of Quantum Technology and Device, Department of Physics, Zhejiang University, Hangzhou, 310027, China.

Zhejiang University of Water Resources and Electric Power, Hangzhou, 310018, China.

出版信息

Sci Rep. 2019 Aug 23;9(1):12307. doi: 10.1038/s41598-019-48662-8.

Abstract

We study the quantum phase transitions in the nickel pnctides, CeNi(AsP) (δ ≈ 0.07-0.22) polycrystalline samples. This series displays the distinct heavy fermion behavior in the rarely studied parameter regime of dilute carrier limit. We systematically investigate the magnetization, specific heat and electrical transport down to low temperatures. Upon increasing the P-content, the antiferromagnetic order of the Ce-4f moment is suppressed continuously and vanishes at x ~ 0.55. At this doping, the temperature dependences of the specific heat and longitudinal resistivity display non-Fermi liquid behavior. Both the residual resistivity ρ and the Sommerfeld coefficient γ are sharply peaked around x. When the P-content reaches close to 100%, we observe a clear low-temperature crossover into the Fermi liquid regime. In contrast to what happens in the parent compound x = 0.0 as a function of pressure, we find a surprising result that the non-Fermi liquid behavior persists over a nonzero range of doping concentration, x < x < 0.9. In this doping range, at the lowest measured temperatures, the temperature dependence of the specific-heat coefficient is logarithmically divergent and that of the electrical resistivity is linear. We discuss the properties of CeNi(AsP) in comparison with those of its 1111 counterpart, CeNi(AsP)O. Our results indicate a non-Fermi liquid phase in the global phase diagram of heavy fermion metals.

摘要

我们研究了镍磷化物CeNi(AsP)(δ≈0.07 - 0.22)多晶样品中的量子相变。该系列在稀载流子极限这一鲜有研究的参数范围内展现出明显的重费米子行为。我们系统地研究了直至低温下的磁化强度、比热和电输运。随着磷含量的增加,Ce - 4f磁矩的反铁磁序被持续抑制,并在x≈0.55时消失。在此掺杂水平下,比热和纵向电阻率的温度依赖性呈现出非费米液体行为。剩余电阻率ρ和索末菲系数γ在x附近都急剧峰值化。当磷含量接近100%时,我们观察到在低温下向费米液体区域的明显转变。与母体化合物x = 0.0随压力变化的情况相反,我们发现一个令人惊讶的结果,即非费米液体行为在非零的掺杂浓度范围x < x < 0.9内持续存在。在这个掺杂范围内,在最低测量温度下,比热系数的温度依赖性呈对数发散,而电阻率的温度依赖性是线性的。我们将CeNi(AsP)的性质与其1111型对应物CeNi(AsP)O的性质进行了比较。我们的结果表明在重费米子金属的全局相图中存在一个非费米液体相。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9184/6707201/e28a8f01e747/41598_2019_48662_Fig1_HTML.jpg

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