The Key Laboratory of Weak-Light Nonlinear Photonics, Ministry of Education, School of Physics and TEDA Institute of Applied Physics, Nankai University, Tianjin 300457, People's Republic of China.
Nanotechnology. 2019 Dec 13;30(50):505201. doi: 10.1088/1361-6528/ab4249. Epub 2019 Sep 6.
Because of extreme three-dimensional field confinement and easy electrically tunability, plasmons in graphene nanostructures are promising candidates for many applications, such as biosensing, photodetectors and modulators. However, up to now, graphene plasmons have been explored mostly on substrates. Scatterers, corrugations and dopants induced by substrates not only add damping to plasmons but also obscure the intrinsic electronic properties of graphene. In this work, the near-field response of surface plasmons of suspended graphene circular resonators is studied with the scattering-type scanning near-field optical microscopy under different excitation wavelengths, λ = 10.653 and 10.22 μm, respectively. Fundamental and higher order breathing plasmon modes are revealed in real-space with the Fermi energy of graphene of only 0.132 eV. Moreover, the direct experimental evidence on near-field electric tuning in suspended graphene resonators is demonstrated by using back-gate tuning. Our work not only provides a foundation to truly understand the properties of electrons inside pure graphene, but shines light on the applications in optoelectronic devices with suspended two-dimensional materials.
由于极端的三维场限制和易于电调谐,石墨烯纳米结构中的等离子体激元是许多应用的有前途的候选者,例如生物传感、光电探测器和调制器。然而,到目前为止,石墨烯等离子体主要在衬底上进行了探索。衬底引起的散射体、波纹和掺杂剂不仅会使等离子体阻尼,还会掩盖石墨烯的固有电子特性。在这项工作中,分别使用 10.653μm 和 10.22μm 的激发波长,通过散射型扫描近场光学显微镜研究了悬空石墨烯圆形谐振器的表面等离子体的近场响应。在石墨烯的费米能仅为 0.132eV 的情况下,在实空间中揭示了基本和更高阶的呼吸等离子体模式。此外,通过背栅调谐证明了悬空石墨烯谐振器中近场电调谐的直接实验证据。我们的工作不仅为真正理解纯石墨烯内部电子的性质提供了基础,而且为具有悬空二维材料的光电设备的应用提供了思路。