Photonics Laboratory, Physics Unit, Tampere University, Tampere, Finland.
Helsinki Institute of Physics, Helsinki University, Helsinki, Finland.
Sci Rep. 2019 Sep 25;9(1):13884. doi: 10.1038/s41598-019-50396-6.
Remote detection of alpha radiation is commonly realised by collecting the light, the radioluminescence, that is produced when alpha particles are stopped in air. Radioluminescence of nitric oxide (NO) is primarily emitted between 200 nm and 300 nm, which makes it possible to use it for remote detection under daylight conditions. Quenching by ambient oxygen and water vapour, however, makes it generally difficult to effectively create NO radioluminescence. We present the detection of intense NO radioluminescence in ambient air under standard indoor lighting conditions using a nitrogen purge. The nitrogen contained NO impurities that were intrinsic to the gas and had not explicitly been added. We study the mechanisms that govern the NO radioluminescence production and introduce a model to describe the dynamics of the process. The level of NO contained in the gas was found to determine how successful a purge can be. We conclude by discussing possible applications of the technique in nitrogen-flushed gloveboxes at nuclear facilities where NO concentration of 100 ppb-1 ppm would be sufficient for efficient optical alpha radiation detection in standard lighting conditions.
α 辐射的远程探测通常通过收集α粒子在空气中停止时产生的光,即辐射发光来实现。一氧化氮(NO)的辐射发光主要在 200nm 和 300nm 之间发射,这使得它可以在日光条件下用于远程探测。然而,环境氧气和水蒸气的猝灭通常使得有效地产生 NO 辐射发光变得困难。我们在标准室内照明条件下使用氮气吹扫,展示了在环境空气中探测强的 NO 辐射发光。氮气中包含的 NO 杂质是气体固有的,而不是特意添加的。我们研究了控制 NO 辐射发光产生的机制,并引入了一个模型来描述该过程的动力学。发现气体中包含的 NO 水平决定了吹扫的成功程度。最后,我们讨论了该技术在核设施中充氮手套箱中的可能应用,在标准照明条件下,100ppb-1ppm 的 NO 浓度就足以实现高效的光学α辐射探测。