Zhang Lixin, Hoogenboom Jacob P, Cook Ben, Kruit Pieter
Department of Imaging Physics, Delft University of Technology, Lorentzweg 1, 2628CJ Delft, The Netherlands.
Struct Dyn. 2019 Sep 27;6(5):051501. doi: 10.1063/1.5117058. eCollection 2019 Sep.
Observing atomic motions as they occur is the dream goal of ultrafast electron microscopy (UEM). Great progress has been made so far thanks to the efforts of many scientists in developing the photoemission sources and beam blankers needed to create short pulses of electrons for the UEM experiments. While details on these setups have typically been reported, a systematic overview of methods used to obtain a pulsed beam and a comparison of relevant source parameters have not yet been conducted. In this report, we outline the basic requirements and parameters that are important for UEM. Different types of imaging modes in UEM are analyzed and summarized. After reviewing and analyzing the different kinds of photoemission sources and beam blankers that have been reported in the literature, we estimate the reduced brightness for all the photoemission sources reviewed and compare this to the brightness in the continuous and blanked beams. As for the problem of pulse broadening caused by the repulsive forces between electrons, four main methods available to mitigate the dispersion are summarized. We anticipate that the analysis and conclusions provided in this manuscript will be instructive for designing an UEM setup and could thus push the further development of UEM.
在原子运动发生时对其进行观测是超快电子显微镜(UEM)的理想目标。多亏了众多科学家在开发用于UEM实验的产生短电子脉冲所需的光发射源和束流消隐器方面所做的努力,到目前为止已经取得了巨大进展。虽然这些装置的细节通常已有报道,但尚未对用于获得脉冲束的方法进行系统概述,也未对相关源参数进行比较。在本报告中,我们概述了对UEM重要的基本要求和参数。对UEM中的不同成像模式进行了分析和总结。在回顾和分析了文献中报道的不同类型的光发射源和束流消隐器后,我们估算了所审查的所有光发射源的折合亮度,并将其与连续束和消隐束中的亮度进行比较。至于由电子间排斥力引起的脉冲展宽问题,总结了四种可用于减轻色散的主要方法。我们预计本手稿中提供的分析和结论将对设计UEM装置具有指导意义,从而推动UEM的进一步发展。