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限制在二维微通道中的自推进活性粒子悬浮液的介观集体运动。

The mesoscopic collective motion of self-propelling active particle suspension confined in two-dimensional micro-channel.

作者信息

Cai Sin-Cen, Shen Yu-Xuan, Io Chong-Wai

机构信息

Many-body System Laboratory, Department of Physics, National Chung-Cheng University, Chiayi 62102, Taiwan, Republic of China. Department of Physics, Republic of China Military Academy, Kaohsiung, 83059, Taiwan, Republic of China.

出版信息

J Phys Condens Matter. 2020 Feb 27;32(9):095101. doi: 10.1088/1361-648X/ab5772. Epub 2019 Nov 13.

Abstract

The mesoscopic collective motion of self-propelling active particle suspension confined in high aspect ratio two-dimensional micro-channel is numerically studied through coupled [Formula: see text] equation by considering background thermal fluctuation, inter-particle interaction, self-propulsion and micro-channel confinement. Both the self-propulsion and micro-channel confinement are the factors driving the system away from equilibrium and sustaining heterogeneous motion. In such system, the propulsion induced particle accumulation around the channel walls is a universal phenomenon with spatial heterogeneity, where large fraction of particles are caged inside the accumulated cluster with local oscillation coexisting with few fast propelling particles in the center region. Although the formation mechanism of the induced accumulation is well studied, post the cluster formation, how the cluster evolves and its dynamical properties is rarely discussed. Based on the merits of [Formula: see text] equation, the dynamical evolution of induced accumulation is revealed by particle trajectories. It is found that the induced accumulation can be dissociated through the slow re-orientation process of few jammed particles. By using the idea of force chain network, how the transverse confinement couples the transverse displacement with the longitudinal displacement is evidenced. It is further verified by the statistical measurement of correlation probability between transverse and longitudinal displacements. The suppressed displacements in both directions is the origin leading to the slow dynamics of cluster evolution. Temporally, within the orientational relaxation time, this system exhibits non-trivial anomalous diffusion under the competition between the counter effects of self-propulsion (enhanced diffusion) and micro-channel confinement (suppressed diffusion). Additionally, by considering the orientational coupling, the deep hysteresis of accumulation has been found even for very weak orientational coupling strength.

摘要

通过耦合[公式:见原文]方程,考虑背景热涨落、粒子间相互作用、自推进和微通道限制,对限制在高纵横比二维微通道中的自推进活性粒子悬浮液的介观集体运动进行了数值研究。自推进和微通道限制都是使系统远离平衡并维持非均匀运动的因素。在这样的系统中,推进导致的粒子在通道壁周围的积累是一种具有空间非均匀性的普遍现象,其中大部分粒子被困在积累的簇内,局部振荡与中心区域少数快速推进的粒子共存。尽管对诱导积累的形成机制已有充分研究,但在簇形成之后,簇如何演化及其动力学性质却很少被讨论。基于[公式:见原文]方程的优点,通过粒子轨迹揭示了诱导积累的动力学演化。发现诱导积累可以通过少数卡住粒子的缓慢重新定向过程解离。利用力链网络的概念,证明了横向限制如何将横向位移与纵向位移耦合起来。横向和纵向位移之间相关概率的统计测量进一步证实了这一点。两个方向上的位移抑制是导致簇演化动力学缓慢的根源。在时间上,在取向弛豫时间内,该系统在自推进(增强扩散)和微通道限制(抑制扩散)的反作用竞争下表现出非平凡的反常扩散。此外,通过考虑取向耦合,即使对于非常弱的取向耦合强度,也发现了积累的深度滞后现象。

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