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准一维微约束下热泳型活性粒子悬浮液的介观聚集行为

Mesoscopic clustering behavior of thermophoretic-type active particle suspension under quasi-one-dimensional microconfinement.

作者信息

Io Chong-Wai, Lee Yu-Yao

机构信息

Many-body System Laboratory, Department of Physics and Center for Nano Bio-Detection, National Chung Cheng University, Chiayi 62102, Taiwan.

出版信息

Phys Rev E. 2021 Jul;104(1-1):014607. doi: 10.1103/PhysRevE.104.014607.

Abstract

We experimentally investigate the mesoscopic clustering behavior of thermophoretic-type active particle suspension under quasi-one-dimensional spatial confinement (high aspect ratio microchannel). The microchannel enhances the viscous dissipation to operate the system in subpropulsion regime. We find that, in the subpropulsion regime, the steady-state configuration of active particle suspension exhibits a transition from homogeneous state to sausagelike clustering bundle located at the channel center, quasiperiodic isolated clusters at the channel center, aperiodic isolated cluster deviated from channel center, and finally to the typical propulsion-induced accumulation around the channel boundary as increasing the excitation laser intensity. The formation of those patterns is under the interplay of outward-pointing mesoscopic scaled thermophoretic force and the applied spatial confinement. The finding of those special patterns can provide some further possibilities of particle manipulation at mesoscopic scale.

摘要

我们通过实验研究了准一维空间限制(高纵横比微通道)下热泳型活性粒子悬浮液的介观聚集行为。微通道增强了粘性耗散,使系统在亚推进状态下运行。我们发现,在亚推进状态下,随着激发激光强度的增加,活性粒子悬浮液的稳态构型呈现出从均匀状态到位于通道中心的香肠状聚集束、通道中心的准周期孤立簇、偏离通道中心的非周期孤立簇,最终到通道边界周围典型的推进诱导聚集的转变。这些模式的形成是向外指向的介观尺度热泳力与施加的空间限制相互作用的结果。这些特殊模式的发现可以为介观尺度下的粒子操纵提供一些进一步的可能性。

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