Spirally deformable soft actuators and their designable helical actuations based on a highly oriented carbon nanotube film.

Spiral configurations and helical curlings of plant tendrils and seed pods are very common in nature. Many researchers have tried to develop spirally deformable actuators to mimic these natural spirals through several approaches, such as preforming helical shapes, processing diagonal stripes and employing anisotropic organic layers. However, these methods are usually complex and time-consuming. Here, we used an efficient method to produce a highly oriented carbon nanotube (CNT) film and develop a series of spirally deformable soft actuators which perform various controllable helical actuations. The actuator consists of a CNT layer with strong anisotropy and a silicone layer. By simply adjusting the orientations of the aligned CNTs, the prepared actuators can accomplish left- or right-handed spiral deformations with different helical forms when driven by electricity. Finite element analyses and simulations were conducted to investigate the mechanism. It is confirmed that it is the anisotropic moduli of the CNT film that regulate the internal stress distributions of the actuators and lead to helical actuations. Moreover, complex actuator designs and functional applications were also carried out. A V-shaped actuator can simultaneously achieve left- and right-handed curling with large angles (630°), which vividly imitates the spiral winding of a tendril. A Y-shaped actuator performed three-dimensional movements, which can manipulate lightweight objects deftly. By virtue of easy preparation and flexible function design, the spirally deformable actuators based on the oriented CNT film will be very promising in artificial muscles and bionic soft robots.